High-performance Polydimethylsiloxane Composites Based on Ordered Three-dimensional PVA-MMT Aerogel Network: Network Structure Regulation and Mechanical Enhancement Mechanism

Zhe-Yu Yang; Long-Jin Huang; Zhao-Qun Shao; Yang Yang; Xia-Yan Cao; Zi-Han Wang; Sheng Cui; Chun-Hua Zhu; Yu Liu

doi:10.1007/s10118-025-3416-5

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High-performance Polydimethylsiloxane Composites Based on Ordered Three-dimensional PVA-MMT Aerogel Network: Network Structure Regulation and Mechanical Enhancement Mechanism

RESEARCH ARTICLE | Updated：2025-10-30

- High-performance Polydimethylsiloxane Composites Based on Ordered Three-dimensional PVA-MMT Aerogel Network: Network Structure Regulation and Mechanical Enhancement Mechanism
- High-performance Polydimethylsiloxane Composites Based on Ordered Three-dimensional PVA-MMT Aerogel Network: Network Structure Regulation and Mechanical Enhancement Mechanism
- 高分子科学（英文） 2025年43卷第11期页码：2171-2184
- Affiliations：
  
  a.State Key Laboratory of Materials-Oriented Chemical Engineering, College of Material Science and Engineering, Nanjing Tech University, Nanjing 211816, China
  b.Institute of Chemical Materials, China Academy of Engineering Physics, Mianyang 621900, China
- Author bio：
  
  cui2002sheng@126.com (S.C.)
  chzhu@caep.cn (C.H.Z.)
  new615@163.com (Y.L.)
- Funds：
  
  This study was financially supported by the National Natural Science Foundation of China (Nos. 21876164 and U2030203) and A Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions.;Electronic supplementary information (ESI) is available free of charge in the online version of this article at http://doi.org/10.1007/s10118-025-3416-5.
- DOI：10.1007/s10118-025-3416-5
  中图分类号：
- 收稿：2025-05-23，
  
  修回：2025-07-11，
  
  录用：2025-07-25，
  
  网络首发：2025-09-24，
  
  纸质出版：2025-11-05
- Accepted：
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Yang, Z. Y.; Huang, L. J.; Shao, Z. Q.; Yang, Y.; Cao, X. Y.; Wang, Z. H.; Cui, S.; Zhu, C. H.; Liu, Y. High-performance polydimethylsiloxane composites based on ordered three-dimensional PVA-MMT aerogel network: network structure regulation and mechanical enhancement mechanism. Chinese J. Polym. Sci. 2025, 43, 2171–2184

Zhe-Yu Yang, Long-Jin Huang, Zhao-Qun Shao, et al. High-performance Polydimethylsiloxane Composites Based on Ordered Three-dimensional PVA-MMT Aerogel Network: Network Structure Regulation and Mechanical Enhancement Mechanism[J]. Chinese Journal of Polymer Science, 2025, 43(11): 2171-2184.
Yang, Z. Y.; Huang, L. J.; Shao, Z. Q.; Yang, Y.; Cao, X. Y.; Wang, Z. H.; Cui, S.; Zhu, C. H.; Liu, Y. High-performance polydimethylsiloxane composites based on ordered three-dimensional PVA-MMT aerogel network: network structure regulation and mechanical enhancement mechanism. Chinese J. Polym. Sci. 2025, 43, 2171–2184 DOI： 10.1007/s10118-025-3416-5.

Zhe-Yu Yang, Long-Jin Huang, Zhao-Qun Shao, et al. High-performance Polydimethylsiloxane Composites Based on Ordered Three-dimensional PVA-MMT Aerogel Network: Network Structure Regulation and Mechanical Enhancement Mechanism[J]. Chinese Journal of Polymer Science, 2025, 43(11): 2171-2184. DOI： 10.1007/s10118-025-3416-5.

摘要

Ordered interconnected three-dimensional PVA-MMT aerogel filler networks with different pore structures were successfully constructed in the PDMS matrix

resulting in significant changes in the mechanical properties of the PDMS composites

including tensile strength

modulus

and elongation at break.

Abstract

To address the poor mechanical properties of polydimethylsiloxane (PDMS) and enhance the understanding of the reinforcement mechanisms of aerogel network structures in rubber matrices

this study reinforced PDMS using an ordered interconnected three-dimensional montmorillonite (MMT) aerogel network. The average pore diameter of the aerogels was successfully reduced from 11.53 μm to 2.51 μm by adjusting the ratio of poly(vinyl alcohol) (PVA) to MMT

via

directional freezing. Changes in the aerogel network were observed in field emission scanning electron microscope (FESEM) images. After vacuum impregnation

the aerogel network structure of the composites was observed using FESEM. Tensile tests indicated that as the pore diameter decreased

the elongation at break of the composites first increased to a peak of 329.61% before decreasing

while the tensile strength and Young's modulus continuously increased to their maximum values of 6.29 MPa and 24.67 MPa

respectively. Meanwhile

FES

EM images of the tensile cracks and fracture surfaces showed that with a reduction in aerogel pore diameter

the degrees of crack deflection and interfacial debonding increased

presenting a rougher fracture surface. These phenomena enable the composites to dissipate substantial energy during tension

thus effectively improving the mechanical strength of the composites. The present work elucidates the bearing of ordered three-dimensional aerogel network structures on the performance of rubber matrices and provides crucial theoretical insights and technical guidance for the creation and optimization of high-performance PDMS-based composites.

关键词

Keywords

references

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