Injection of a Self-propelled Polymer into a Small Circular Cavity

Chao Wang; Yan-Li Zhou; Xiao Yang; Fan Wu; Meng-Bo Luo

doi:10.1007/s10118-024-3103-y

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Injection of a Self-propelled Polymer into a Small Circular Cavity

RESEARCH ARTICLE | Updated：2024-05-11

- Injection of a Self-propelled Polymer into a Small Circular Cavity
- Injection of a Self-propelled Polymer into a Small Circular Cavity
- 高分子科学（英文版） 2024年42卷第6期页码：886-894
- Affiliations：
  
  a.Department of Physics, Taizhou University, Taizhou 318000, China
  b.Department of Physics, Zhejiang University, Hangzhou 310027, China
- Author bio：
  
  chaowang0606@126.com
- Funds：
  
  This work was financially supported by the Zhejiang Provincial Natural Science Foundation of China (No. LY20A040004) and by the National Natural Science Foundation of China (Nos. 11604232 and 11974305).
- DOI：10.1007/s10118-024-3103-y
  中图分类号：
- 收稿：2023-12-30，
  
  修回：2024-1-31，
  
  录用：2024-2-10，
  
  网络首发：2024-03-29，
  
  纸质出版：2024-06-01
- Accepted：
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Wang, C.; Zhou, Y. L.; Yang, X.; Wu, F.; Luo, M. B. Injection of a self-propelled polymer into a small circular cavity. Chinese J. Polym. Sci. 2024, 42, 886–894

Chao Wang, Yan-Li Zhou, Xiao Yang, et al. Injection of a Self-propelled Polymer into a Small Circular Cavity[J]. Chinese Journal of Polymer Science, 2024, 42(6): 886-894.
Wang, C.; Zhou, Y. L.; Yang, X.; Wu, F.; Luo, M. B. Injection of a self-propelled polymer into a small circular cavity. Chinese J. Polym. Sci. 2024, 42, 886–894 DOI： 10.1007/s10118-024-3103-y.

Chao Wang, Yan-Li Zhou, Xiao Yang, et al. Injection of a Self-propelled Polymer into a Small Circular Cavity[J]. Chinese Journal of Polymer Science, 2024, 42(6): 886-894. DOI： 10.1007/s10118-024-3103-y.

摘要

Under the driving of the tangential active force

the part of polymer inside the circular cavity adopts random coil configuration at small polymer rigidity and spiral configuration at moderate or large polymer rigidity

resulting that the injection time shows nonmonotonouse dependence on the polymer rigidity.

Abstract

The injection of a polymer chain into a small circular cavity under tangential self-propelled force is studied by using Langevin dynamics simulation. Results indicate that the injection dynamics of the active polymer shows strong correlation with the polymer conformation inside the cavity depending on the polymer rigidity (

). The injection time

varies nonmonotonously with increasing

and reaches its minimum at

. When

is small (

)

the polymer is nearly ran

dom coil in the cavity

and spends a long time at the final stage of the injection process due to the large repulsion between monomers inside the cavity. When

is moderate (

)

the part of polymer inside the cavity forms spiral configuration under the tangential active force

and the whole polymer moves synchronously with a constant velocity during the injection process

leading to a small injection time. When

is large (

)

the polymer is nearly straight at the initial stage of the injection process

and takes a long time to bend itself

leading to a large injection time.

关键词

Keywords

references

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