Synergistic Optimization of Toughness and EMI Shielding Properties in Rigid Polyurethane Composites by Designing Ring Structures on the Surface of Carbon Fibers

Yi-Long Zhou; Wei-Wei Li; Hui-Xin Liu; Kai-Yuan Pei; Shi-Ting Li

doi:10.1007/s10118-023-2999-y

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Synergistic Optimization of Toughness and EMI Shielding Properties in Rigid Polyurethane Composites by Designing Ring Structures on the Surface of Carbon Fibers

RESEARCH ARTICLE | Updated：2023-11-27

- Synergistic Optimization of Toughness and EMI Shielding Properties in Rigid Polyurethane Composites by Designing Ring Structures on the Surface of Carbon Fibers
- Synergistic Optimization of Toughness and EMI Shielding Properties in Rigid Polyurethane Composites by Designing Ring Structures on the Surface of Carbon Fibers
- 高分子科学（英文版） 2023年41卷第12期页码：1958-1968
- Affiliations：
  
  School of Materials Science and Chemical Engineering, Ningbo University, Ningbo 315211, China
- Author bio：
  
  liweiwei@nbu.edu.cn
- Funds：
  
  This work was financially supported by Ningbo Natural Science Foundation (No. 2022J103).
- DOI：10.1007/s10118-023-2999-y
  中图分类号：
- 收稿：2023-02-23，
  
  修回：2023-4-17，
  
  录用：2023-5-4，
  
  网络首发：2023-06-12，
  
  纸质出版：2023-12-01
- Accepted：
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Zhou, Y. L.; Li, W. W.; Liu, H. X.; Pei, K. Y.; Li, S. T. Synergistic optimization of toughness and EMI shielding properties in rigid polyurethane composites by designing ring structures on the surface of carbon fibers. Chinese J. Polym. Sci. 2023, 41, 1958–1968

Yi-Long Zhou, Wei-Wei Li, Hui-Xin Liu, et al. Synergistic Optimization of Toughness and EMI Shielding Properties in Rigid Polyurethane Composites by Designing Ring Structures on the Surface of Carbon Fibers[J]. Chinese Journal of Polymer Science, 2023, 41(12): 1958-1968.
Zhou, Y. L.; Li, W. W.; Liu, H. X.; Pei, K. Y.; Li, S. T. Synergistic optimization of toughness and EMI shielding properties in rigid polyurethane composites by designing ring structures on the surface of carbon fibers. Chinese J. Polym. Sci. 2023, 41, 1958–1968 DOI： 10.1007/s10118-023-2999-y.

Yi-Long Zhou, Wei-Wei Li, Hui-Xin Liu, et al. Synergistic Optimization of Toughness and EMI Shielding Properties in Rigid Polyurethane Composites by Designing Ring Structures on the Surface of Carbon Fibers[J]. Chinese Journal of Polymer Science, 2023, 41(12): 1958-1968. DOI： 10.1007/s10118-023-2999-y.

摘要

We designed and prepared the ring-shaped zinc coating on carbon fiber surface

which improved the interfacial properties between fibers and the matrix and resulted in the enhanced toughness of the composites. The synergistic effect of porous structure and conductive network caused by ring-shaped zinc decorated carbon fibers in the RPU matrix made the composites exhibited the satisfactory electrical conductivity and EMI shielding properties.

Abstract

How to achieve both toughness and enhanced electromagnetic interference shielding effectiveness (EMI SE) of carbon fibers (CFs) reinforced rigid polyurethane (RPU) composites is a significative challenge at present. In this work

a ring-shaped zinc coating was deposited on the short CFs by electrodeposition technique. It is expected to improve the interfacial properties between the fibers and the resin matrix as well as enhance the EMI shielding properties of the composites by changing the surface morphology and roughness of the fibers. Results showed that the surface free energy of the ring-shaped zinc modified carbon fibers (RS-CFs) increased from 49.0 mJ/m

to 53.2 mJ/m

indicating that the surface roughness and wettability of the CFs were effectively improved. In comparison with the pristine short carbon fibers/rigid polyurethane (CFs/RPU) composites

tensile strength and tensile toughness of RS-CFs modified composites were increased by 27.1% and 121.4%

respectively. In addition

the bending and impact strengths of RS-CFs reinforced RPU composites were also improved. Notably

the electrical conductivity of RS-CFs/RPU composites reached 1.2×10

−5

S/m

which was much higher than that of CFs/RPU composites at 1.4×10

−10

S/m. Moreover

the EMI SE of the modified composites reached 22 dB

which was 152.9% higher than that of CFs/RPU composites. The enhanced electrical conductivity and EMI shielding properties of the composites could be attributed to the synergistic effect of the porous structure in the RPU matrix and the CFs modified by the metal coating.

关键词

Keywords

references

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Effects of Different Nucleating Agents, Annealing and Pre-stretching Process on the Crystallinity and Mechanical Properties of Poly(butylene carbonate)

Advancing the Thin-film Mechanics of Conjugated Polymers: Characterization, Modulation, and Innovation

Enhanced Mechanical Properties and Prolonged Recovery Onset Period of Timed Shape Memory Hydrogels via Hydrophobic Interaction

Durable Anti-fogging and Abrasion-resistant Coatings Based on Polyoxometalates-Hydrophilic Resin Composites with Enhanced Cohesion and Adhesion