Enhanced Adhesion Properties of Polymer-Metal Interfaces <italic style="font-style: italic">via</italic> Nano-injection Molding: A Study on Molecular Kinematic Mechanisms

Hong-Chen Li; Dong-Lei Liu; Xin Luo; Tian Yuan; Kai Zhan; Jing Gan

doi:10.1007/s10118-023-2906-6

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Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms

RESEARCH ARTICLE | Updated：2023-05-26

- Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms
- Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms
- 高分子科学（英文版） 2023年41卷第6期页码：981-993
- Affiliations：
  
  School of Advanced Manufacturing, Nanchang University, Nanchang 330031, China
- Author bio：
  
  dlliu@ncu.edu.cn
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (No. 52165046). We thank the anonymous reviewers, whose comments have helped improve the presentation of our work.
- DOI：10.1007/s10118-023-2906-6
  中图分类号：
- 收稿：2022-08-24，
  
  修回：2022-10-21，
  
  录用：2022-11-15，
  
  网络首发：2023-01-31，
  
  纸质出版：2023-06-01
- Accepted：
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Li, H. C.; Liu, D. L.; Luo, X.; Yuan, T.; Zhan, K.; Gan, J. Enhanced adhesion properties of polymer-metal interfaces via nano-injection molding: a study on molecular kinematic mechanisms. Chinese J. Polym. Sci. 2023, 41, 981–993

Hong-Chen Li, Dong-Lei Liu, Xin Luo, et al. Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms[J]. Chinese Journal of Polymer Science, 2023, 41(6): 981-993. DOI: 10.1007/s10118-023-2906-6.
Li, H. C.; Liu, D. L.; Luo, X.; Yuan, T.; Zhan, K.; Gan, J. Enhanced adhesion properties of polymer-metal interfaces via nano-injection molding: a study on molecular kinematic mechanisms. Chinese J. Polym. Sci. 2023, 41, 981–993 DOI： 10.1007/s10118-023-2906-6.

Hong-Chen Li, Dong-Lei Liu, Xin Luo, et al. Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms[J]. Chinese Journal of Polymer Science, 2023, 41(6): 981-993. DOI: 10.1007/s10118-023-2906-6. DOI：

摘要

In this study

three kinds of PPS-Al

PPS-Cu and PPS-Fe interfacial models with pyramidal nano-slots were modeled. The multiple-anchor-point slipping phenomenon was in nano-injection molding revealed. And the molecular kinematic mechanisms of polymer-metal interface interactive were studied.

Abstract

Nano-injection molding enables the formation of nano-scale anchors to connect heterogeneous material surfaces to achieve the required mechanical properties. In this work

polyphenylene sulfide (PPS)

aluminum (Al)

copper (Cu)

and iron (Fe) were selected as candidate polymer and metal materials. Three kinds of polymer-metal interfacial models with pyramidal nano-slots were modeled. The molecular dynamics simulations were launched to investigate the adhesion properties and molecular kinematic mechanisms of heterogeneous interfaces in nano-injection molding. Results showed that the wall-slipping behavior of PPS at the interface slot was obvious

it was easy to form multiple-anchor-points in the central area of substrates

and these anchor points were easily slipping along the wall

different from the de Gennes model. The atomic lattice and atomic band gap of metal affected the adhesion strength. The BCC lattice of Fe was more suitable for nano-injection molding process than the FCC lattice of Al and Cu. The filling rate

interfacial energy

the tensile and shear failures data revealed that the interfacial adhesion performances decreased according to the following order

Fe-PPS

Cu-PPS and Al-PPS components

respectively

and the interface failure mode was closely related to the stress loading mode.

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references

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Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms

Enhanced Adhesion Properties of Polymer-Metal Interfaces via Nano-injection Molding: A Study on Molecular Kinematic Mechanisms

DOI：10.1007/s10118-023-2906-6

摘要

Abstract

关键词

Keywords

references