Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding, Electrothermal and Solarthermal Performances

Ming-Ke Xu; Xin-Jie Luo; Hao-Bin Zhang; Yu Zhang; Lu-Lu Li; Xin-Feng Zhou; Zhong-Zhen Yu

doi:10.1007/s10118-022-2813-2

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Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding, Electrothermal and Solarthermal Performances

RESEARCH ARTICLE | Updated：2023-01-06

- Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding, Electrothermal and Solarthermal Performances
- Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding, Electrothermal and Solarthermal Performances
- 高分子科学（英文版） 2023年41卷第2期页码：267-277
- Affiliations：
  
  a.Beijing Key Laboratory of Advanced Functional Polymer Composites, Beijing University of Chemical Technology, Beijing 100029, China
  b.State Key Laboratory of Organic-Inorganic Composites, College of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, China
- Author bio：
  
  zhanghaobin@mail.buct.edu.cn (H.B.Z.)
  yuzz@mail.buct.edu.cn (Z.Z.Y.)
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (Nos. 51922020 and 52090034), and the Fundamental Research Funds for the Central Universities (Nos. BHYC1707B and XK1802-2).;Electronic supplementary information (ESI) is available free of charge in the online version of this article at http://doi.org/10.1007/s10118-022-2813-2.
- DOI：10.1007/s10118-022-2813-2
  中图分类号：
- 收稿：2022-05-07，
  
  修回：2022-5-19，
  
  录用：2022-6-10，
  
  网络首发：2022-09-26，
  
  纸质出版：2023-02-01
- Accepted：
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Xu, M. K.; Luo, X. J.; Zhang, H. B.; Zhang, Y.; Li, L. L.; Zhou, X. F.; Yu, Z. Z. Multifunctional waterborne polyurethane nanocomposite films with remarkable electromagnetic interference shielding, electrothermal and solarthermal performances. Chinese J. Polym. Sci. 2023, 41, 267–277

Ming-Ke Xu, Xin-Jie Luo, Hao-Bin Zhang, et al. Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding, Electrothermal and Solarthermal Performances[J]. Chinese Journal of Polymer Science, 2023, 41(2): 267-277.
Xu, M. K.; Luo, X. J.; Zhang, H. B.; Zhang, Y.; Li, L. L.; Zhou, X. F.; Yu, Z. Z. Multifunctional waterborne polyurethane nanocomposite films with remarkable electromagnetic interference shielding, electrothermal and solarthermal performances. Chinese J. Polym. Sci. 2023, 41, 267–277 DOI： 10.1007/s10118-022-2813-2.

Ming-Ke Xu, Xin-Jie Luo, Hao-Bin Zhang, et al. Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding, Electrothermal and Solarthermal Performances[J]. Chinese Journal of Polymer Science, 2023, 41(2): 267-277. DOI： 10.1007/s10118-022-2813-2.

摘要

Multifunctional MXene/ST-ZnO/WPU nanocomposite films exhibit excellent EMI shielding performances

satisfactory Joule heating and solar-thermal conversion properties.

Abstract

To impart polymers with high electrical conductivity and satisfactory electromagnetic interference shielding efficiency

it is crucial to efficiently construct interconnecting networks of conductive nanofillers in polymer matrices. Herein

on the basis of the three-dimensional (3D) skeleton and volume-exclusion effect of silane-modified tetra-needle ZnO (ST-ZnO) whiskers and the high conductivity of two-dimensional MXene nanosheets

multifunctional MXene/ST-ZnO/waterborne polyurethane (MTW) nanocomposite films are fabricated by coating of MXene on ST-ZnO followed by compounding with waterborne polyurethane. The 3D four-needles of the whiskers facilitate the formation of an interconnecting network in the waterborne polyurethane matrix

while the coating of MXene efficiently makes the interconnecting network of the whiskers conductive at a low amount of the MXene. The resultant MTW ternary nanocomposite film exhibits not only a high electrical conductivity of 4.8×10

S/m

but also an excellent electromagnetic interference shielding effectiveness of over 70 dB in the X-band at a low thickness of 100 μm. In addition

the ternary film also exhibits outstanding Joule heating performances with an equilibrium temperature of 113 °C at a low driving voltage of 3 V. The multifunctional nanocomposite films are promising for applications in portable and wearable electronics and flexible electromagnetic interference shielding devices.

关键词

Keywords

references

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