Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)

Liang-Qing Zhang; Shu-Gui Yang; Jing-Han Zhang; Ke-Peng Zhong; Zhong-Guo Zhao; Yan-Hui Chen; Jun Lei; Qiu-Yu Zhang; Zhong-Ming Li

doi:10.1007/s10118-022-2672-x

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Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)

RESEARCH ARTICLE | Updated：2022-03-23

- Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)
- Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)
- Chinese Journal of Polymer Science 2022年40卷第3期页码：290-298
- Affiliations：
  
  a.College of Material Science and Engineering, Xi’an University of Science and Technology, Xi’an 710054, China
  b.State Key Laboratory for Mechanical Behaviour of Materials, Shaanxi International Research Center for Soft Materials, Xi’an Jiaotong University, Xi’an 710049, China
  c.School of Chemistry and Chemical Engineering, Shaanxi Key Laboratory of Macromolecular Science and Technology, Key Laboratory of Special Functional and Smart Polymer Materials of Ministry of Industry and Information Technology, Northwestern Polytechnical University, Xi’an 710072, China
  d.National and Local Engineering Laboratory for Slag Comprehensive Utilization and Environment Technology, School of Materials Science and Engineering, Shaanxi University of Technology, Hanzhong 723000, China
  e.College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu 610065, China
- Author bio：
  
  yanhuichen@nwpu.edu.cn
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (Nos. 21676217, 52003215, 21978240 and 52003219), Youth Project of Basic Research Program of Natural Science in Shaanxi Province (No. 2020JQ-179) the Fundamental Research Funds for the Central Universities (Nos. 3102018AX004 and 3102017jc01001), and the Open Testing Foundation of the Analytical & Testing Center of Northwestern Polytechnical University (No. 2020T020). The authors thank Shanghai Synchrotron Radiation Facility (SSRF) for supporting the X-ray measurements.
- DOI：10.1007/s10118-022-2672-x
  中图分类号：
- 收稿：2021-08-09，
  
  修回：2021-11-2，
  
  录用：2021-11-23，
  
  网络首发：2022-01-15，
  
  纸质出版：2022-03-01
- Accepted：
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Zhang, L. Q.; Yang, S. G.; Zhang, J. H.; Zhong, K. P.; Zhao, Z. G.; Chen, Y. H.; Lei, J.; Zhang, Q. Y.; Li, Z. M. Insight into the excellent tribological performance of highly oriented poly(phenylene sulfide). Chinese J. Polym. Sci. 2022, 40, 290–298

Liang-Qing Zhang, Shu-Gui Yang, Jing-Han Zhang, et al. Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)[J]. Chinese Journal of Polymer Science, 2022, 40(3): 290-298.
Zhang, L. Q.; Yang, S. G.; Zhang, J. H.; Zhong, K. P.; Zhao, Z. G.; Chen, Y. H.; Lei, J.; Zhang, Q. Y.; Li, Z. M. Insight into the excellent tribological performance of highly oriented poly(phenylene sulfide). Chinese J. Polym. Sci. 2022, 40, 290–298 DOI： 10.1007/s10118-022-2672-x.

Liang-Qing Zhang, Shu-Gui Yang, Jing-Han Zhang, et al. Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)[J]. Chinese Journal of Polymer Science, 2022, 40(3): 290-298. DOI： 10.1007/s10118-022-2672-x.

摘要

Abstract

Achieving low friction and wear of poly(phenylene sulfide) (PPS) without using fillers or blending is a challenging task

but one of considerable practical importance. Here we describe how neat PPS with high tribological performance is achieved by manipulating processing parameters (pressure

flow and temperature). The key to achieving high tribological performance is comparatively high molecular chain orientation

realized in neat PPS

at high shear rates and low pressure. The friction coefficient and wear rate are as low as ~0.3 and ~10

‒6

·N

‒1

·m

‒1

respectively

which break the record for neat PPS. These values are even better than those for PPS-based blends and comparable to PPS composites. Further studies show

for the first time

that wear rate decreases exponentially with increasing molecular chain orientation

prompting us to revise the classical Archard’s law by including the effect of molecular chain orientation. These ﬁndings open the possibility of using neat PPS in highly demanding tribological applications.

关键词

Keywords

references

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