Achieving Efficient Thick Film All-polymer Solar Cells Using a Green Solvent Additive

Zhen-Ye Li; Wen-Kai Zhong; Lei Ying; Ning Li; Feng Liu; Fei Huang; Yong Cao

doi:10.1007/s10118-020-2356-3

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Achieving Efficient Thick Film All-polymer Solar Cells Using a Green Solvent Additive

ARTICLE | Updated：2019-11-27

- Achieving Efficient Thick Film All-polymer Solar Cells Using a Green Solvent Additive
- Achieving Efficient Thick Film All-polymer Solar Cells Using a Green Solvent Additive
- Chinese Journal of Polymer Science 2020年38卷第4期页码：323-331
- Affiliations：
  
  a.Institute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, China
  b.South China Institute of Collaborative Innovation, Dongguan 523808, China
  c.Institute of Materials for Electronics and Energy Technology (i-MEET), FAU Erlangen-Nürnberg, 91058 Erlangen, Germany
  d.Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China
- Author bio：
  
  msleiying@scut.edu.cn (L.Y.)
  msfhuang@scut.edu.cn (F.H.)
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (Nos. 21822505, 91633301, 51673069, and 21520102006), Program for Science and Technology Development of Dongguan (No. 2019622163009), and the Dongguan Innovative Research Team Program (No. 2018607201002). Portions of this research used the resources of beamline 7.3.3 and 11.0.1.2 at Advanced Light Source, Materials Science Division, The Molecular Foundry, Lawrence Berkeley National Laboratory, which was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231.
- DOI：10.1007/s10118-020-2356-3
  中图分类号：
- 收稿：2019-08-01，
  
  修回：2019-9-5，
  
  录用：2019-9-16，
  
  网络首发：2019-11-27，
  
  纸质出版：2020-04
- Accepted：
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Li, Z. Y.; Zhong, W. K.; Ying, L.; Li, N.; Liu, F.; Huang, F.; Cao, Y. Achieving efficient thick film all-polymer solar cells using a green solvent additive. Chinese J. Polym. Sci. 2020, 38, 323–331

Zhen-Ye Li, Wen-Kai Zhong, Lei Ying, et al. Achieving Efficient Thick Film All-polymer Solar Cells Using a Green Solvent Additive[J]. Chinese Journal of Polymer Science, 2020, 38(4): 323-331.
Li, Z. Y.; Zhong, W. K.; Ying, L.; Li, N.; Liu, F.; Huang, F.; Cao, Y. Achieving efficient thick film all-polymer solar cells using a green solvent additive. Chinese J. Polym. Sci. 2020, 38, 323–331 DOI： 10.1007/s10118-020-2356-3.

Zhen-Ye Li, Wen-Kai Zhong, Lei Ying, et al. Achieving Efficient Thick Film All-polymer Solar Cells Using a Green Solvent Additive[J]. Chinese Journal of Polymer Science, 2020, 38(4): 323-331. DOI： 10.1007/s10118-020-2356-3.

摘要

Abstract

Advances in organic photovoltaic technologies have been geared toward industrial high-throughput printing manufacturing

which requires insensitivity of photovoltaic performance regarding to the light-harvesting layer thickness. However

the thickness of light-harvesting layer for all polymer solar cells (all-PSCs) is often limited to about 100 nm due to the dramatically decreased fill factor upon increasing film thickness

which hampers the light harvesting capability to increase the power conversion efficiency

and is unfavorable for fabricating large-area devices. Here we demonstrate that by tuning the bulk heterojunction morphology using a non-halogenated solvent

cyclopentyl methyl ether

in the presence of a green solvent additive of dibenzyl ether

the power conversion efficiency of all-PSCs with photoactive layer thicknesses of over 500 nm reached an impressively high value of 9%. The generic applicability of this green solvent additive to boost the power conversion efficiency of thick-film devices is also validated in various bulk heterojunction active layer systems

thus representing a promising approach for the fabrication of all-PSCs toward industrial production

as well as further commercialization.

关键词

Keywords

references

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