Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels

Jie-xin Liao; Jia-he Huang; Tao Wang; Wei-xiang Sun; Zhen Tong

doi:10.1007/s10118-017-1991-9

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Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels

Papers | Updated：2021-02-18

- Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels
- Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels
- Chinese Journal of Polymer Science 2017年35卷第10期页码：1297-1306
- Affiliations：
  
  a.Research Institute of Materials Science, South China University of Technology, Guangzhou 510640, China
  b.State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, China
- Author bio：
  
  Tao Wang (王涛), E-mail:fetwang@scut.edu.cn
  Zhen Tong (童真), E-mail:mcztong@scut.edu.cn
- Funds：
  
  the National Natural Science Foundation of China(51573060);the National Natural Science Foundation of China(21427805);the Pearl River S & T Nova Program of Guangzhou(201710010146);Supplementary material is available in the online version of this article at http://dx.doi.org/10.1007/s10118-017-1991-9.
- DOI：10.1007/s10118-017-1991-9
  中图分类号：
- 收稿：2017-04-26，
  
  修回：2017-5-30，
  
  录用：2017-6-6，
  
  纸质出版：2017-10-05
- Accepted：
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Jie-xin Liao, Jia-he Huang, Tao Wang, 等. Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels[J]. Chinese Journal of Polymer Science, 2017,35(10):1297-1306.

Jie-xin Liao, Jia-he Huang, Tao Wang, et al. Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels[J]. Chinese Journal of Polymer Science, 2017, 35(10): 1297-1306.
Jie-xin Liao, Jia-he Huang, Tao Wang, 等. Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels[J]. Chinese Journal of Polymer Science, 2017,35(10):1297-1306. DOI： 10.1007/s10118-017-1991-9.

Jie-xin Liao, Jia-he Huang, Tao Wang, et al. Rapid Shape Memory and pH-modulated Spontaneous Actuation of Dopamine Containing Hydrogels[J]. Chinese Journal of Polymer Science, 2017, 35(10): 1297-1306. DOI： 10.1007/s10118-017-1991-9.

摘要

Abstract

The dopamine containing hydrogels with rapid responsive shape memory capability were synthesized by a one-pot method. The temporary shape of hydrogel was fixed within 20 s in NaOH solution by the tris-complex crosslinking of metal-ligand complex between Fe

ions and catechol groups

while the permanent shape was recovered completely in HCl solution within 60 s upon the change from tris-complex to mono-complex. The hydrogel showed unique spontaneous actuation behavior. It could curl spontaneously without further external force deformation when immersed in NaOH solution again after the first shape recovery in HCl solution. This might be attributed to the competitive result of swelling and additional tris-complex crosslinking formation when immersed in NaOH solution. In addition

the hydrogels also had proper modulus

elongation ratio and tensile strength. Such hydrogel provides a new candidate material for designing soft actuators and robots modulated with spontaneous actuating.

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Keywords

references

Q. Zhao , H.J. Qi , T. Xie . Prog. Polym. Sci. , 2015 . 49-50 ( 1 ): 79 http://www.sciencedirect.com/science/article/pii/S0079670015000477 http://www.sciencedirect.com/science/article/pii/S0079670015000477 , .

M.D. Hager , S. Bode , C. Weber , U.S. Schubert . Prog. Polym. Sci. , 2015 . 49-50 ( 1 ): 3 http://www.sciencedirect.com/science/article/pii/S0079670015000489 http://www.sciencedirect.com/science/article/pii/S0079670015000489 , .

Y. Osada , A. Matsuda . Nature , 1995 . 376 ( 6537 ): 219 http://europepmc.org/abstract/med/7617029 http://europepmc.org/abstract/med/7617029 , .

W. Lu , X. Le , J. Zhang , Y. Huang , T. Chen . Chem. Soc. Rev. , 2017 . 46 ( 5 ): 1284 DOI: 10.1039/C6CS00754F http://doi.org/10.1039/C6CS00754F .

M. Behl , M.Y. Razzaq , A. Lendlein . Adv. Mater. , 2010 . 22 ( 31 ): 3388 DOI: 10.1002/adma.200904447 http://doi.org/10.1002/adma.200904447 .

S. Chaterji , I.K. Kwon , K. Park . Prog. Polym. Sci. , 2007 . 32 ( 8-9 ): 1083 DOI: 10.1016/j.progpolymsci.2007.05.018 http://doi.org/10.1016/j.progpolymsci.2007.05.018 .

Z. Ren , Y. Zhang , Y. Li , B. Xu , W. Liu . J. Mater. Chem. B , 2015 . 3 ( 30 ): 6347 DOI: 10.1039/C5TB00781J http://doi.org/10.1039/C5TB00781J .

X. Lu , C.Y. Chan , K.I. Lee , P.F. Ng , B. Fei , J.H. Xin , J. Fu . J. Mater. Chem. B , 2014 . 2 ( 43 ): 7631 DOI: 10.1039/C4TB01289E http://doi.org/10.1039/C4TB01289E .

W. Nan , W. Wang , H. Gao , W. Liu . Soft Matter , 2013 . 9 ( 1 ): 132 DOI: 10.1039/C2SM26918J http://doi.org/10.1039/C2SM26918J .

Y. Han , T. Bai , W. Liu . Sci. Rep. , 2014 . 4 ( 1 ): 5815 .

N. Annabi , A. Tamayol , J.A. Uquillas , M. Akbari , L.E. Bertassoni , C. Cha , G. Camci-Unal , M.R. Dokmeci , N.A. Peppas , A. Khademhosseini . Adv. Mater. , 2014 . 26 ( 1 ): 85 DOI: 10.1002/adma.201303233 http://doi.org/10.1002/adma.201303233 .

L. Ionov . Mater. Today , 2014 . 17 ( 10 ): 494 DOI: 10.1016/j.mattod.2014.07.002 http://doi.org/10.1016/j.mattod.2014.07.002 .

J. Huang , L. Zhao , T. Wang , W. Sun , Z. Tong . ACS Appl. Mater. Interfaces , 2016 . 8 ( 19 ): 12384 DOI: 10.1021/acsami.6b00867 http://doi.org/10.1021/acsami.6b00867 .

X. Qi , X. Yao , S. Deng , T. Zhou , Q. Fu . J. Mater. Chem. A , 2014 . 2 ( 7 ): 2240 DOI: 10.1039/C3TA14340F http://doi.org/10.1039/C3TA14340F .

A. Yasin , W. Zhou , H. Yang , H. Li , Y. Chen , X. Zhang . Macromol. Rapid Commun. , 2015 . 36 ( 9 ): 845 DOI: 10.1002/marc.201400698 http://doi.org/10.1002/marc.201400698 .

H. Meng , J. Zheng , X. Wen , Z. Cai , J. Zhang , T. Chen . Macromol. Rapid Commun. , 2015 . 36 ( 6 ): 533 DOI: 10.1002/marc.v36.6 http://doi.org/10.1002/marc.v36.6 .

K. Miyamae , M. Nakahata , Y. Takashima , A. Harada . Angew. Chem. Int. Ed. , 2015 . 54 ( 31 ): 8984 DOI: 10.1002/anie.201502957 http://doi.org/10.1002/anie.201502957 .

X. Le , W. Lu , H. Xiao , L. Wang , C. Ma , J. Zhang , Y. Huang , T. Chen . ACS Appl. Mater. Interfaces , 2017 . 9 ( 10 ): 9038 DOI: 10.1021/acsami.7b00169 http://doi.org/10.1021/acsami.7b00169 .

M. Wei , M. Zhan , D. Yu , H. Xie , M. He , K. Yang , Y. Wang . ACS Appl. Mater. Interfaces , 2015 . 7 ( 4 ): 2585 DOI: 10.1021/am507575z http://doi.org/10.1021/am507575z .

Y. Chen , L. Peng , T. Liu , Y. Wang , S. Shi , H. Wang . ACS Appl. Mater. Interfaces , 2016 . 8 ( 40 ): 27199 DOI: 10.1021/acsami.6b08374 http://doi.org/10.1021/acsami.6b08374 .

Z. Li , W. Lu , T. Ngai , X. Le , J. Zheng , N. Zhao , Y. Huang , X. Wen , J. Zhang , T. Chen . Polym. Chem. , 2016 . 7 ( 34 ): 5343 DOI: 10.1039/C6PY01112H http://doi.org/10.1039/C6PY01112H .

X. Le , W. Lu , J. Zheng , D. Tong , N. Zhao , C. Ma , H. Xiao , J. Zhang , Y. Huang , T. Chen . Chem. Sci. , 2016 . 7 ( 11 ): 6715 DOI: 10.1039/C6SC02354A http://doi.org/10.1039/C6SC02354A .

H. Xiao , W. Lu , X. Le , C. Ma , Z. Li , J. Zheng , J. Zhang , Y. Huang , T. Chen . Chem. Commun. , 2016 . 52 ( 90 ): 13292 DOI: 10.1039/C6CC06813H http://doi.org/10.1039/C6CC06813H .

B. Xu , Y. Li , F. Gao , X. Zhai , M. Sun , W. Lu , Z. Cao , W. Liu . ACS Appl. Mater. Interfaces , 2015 . 7 ( 30 ): 16865 DOI: 10.1021/acsami.5b05074 http://doi.org/10.1021/acsami.5b05074 .

L. Zhao , J. Huang , T. Wang , W. Sun , Z. Tong . Macromol. Mater. Eng. , 2017 . 302 ( 2 ): 1600359 DOI: 10.1002/mame.v302.2 http://doi.org/10.1002/mame.v302.2 .

Y. Geng , X.Y. Lin , P. Pan , G. Shan , Y. Bao , Y. Song , Z.L. Wu , Q. Zheng . Polymer , 2016 . 100 60 DOI: 10.1016/j.polymer.2016.08.022 http://doi.org/10.1016/j.polymer.2016.08.022 .

R.D. Harris , J.T. Auletta , S.A.M. Motlagh , M.J. Lawless , N.M. Perri , S. Saxena , L.M. Weiland , D.H. Waldeck , W.W. Clark , T.Y. Meyer . ACS Macro Lett. , 2013 . 2 ( 12 ): 1095 DOI: 10.1021/mz4004997 http://doi.org/10.1021/mz4004997 .

J. Yang , M.A. Cohen Stuart , M. Kamperman . Chem. Soc. Rev. , 2014 . 43 ( 24 ): 8271 DOI: 10.1039/C4CS00185K http://doi.org/10.1039/C4CS00185K .

S.W. Taylor , J.H. Waite . Inorg. Chem. , 1994 . 33 ( 25 ): 5819 DOI: 10.1021/ic00103a032 http://doi.org/10.1021/ic00103a032 .

Y. Liu , K. Ai , L. Lu . Chem. Rev. , 2014 . 114 ( 9 ): 5057 DOI: 10.1021/cr400407a http://doi.org/10.1021/cr400407a .

J. Sedó , J. Saiz-Poseu , F. Busqué , D. Ruiz-Molina . Adv. Mater. , 2013 . 25 ( 5 ): 653 DOI: 10.1002/adma.201202343 http://doi.org/10.1002/adma.201202343 .

M. Dong , S. Liu , L. Tan , L. Cen , G. Fu . Chinese J. Polym. Sci. , 2016 . 34 ( 5 ): 637 DOI: 10.1007/s10118-016-1783-7 http://doi.org/10.1007/s10118-016-1783-7 .

M. Krogsgaard , M.A. Behrens , J.S. Pedersen , H. Birkedal . Biomacromolecules , 2013 . 14 ( 2 ): 297 DOI: 10.1021/bm301844u http://doi.org/10.1021/bm301844u .

S. Hou , P.X. Ma . Chem. Mater. , 2015 . 27 ( 22 ): 7627 DOI: 10.1021/acs.chemmater.5b02839 http://doi.org/10.1021/acs.chemmater.5b02839 .

N. Holten-Andersen , M.J. Harrington , H. Birkedal , B.P. Lee , P.B. Messersmith , K.Y.C. Lee , J.H. Waite . P. Natl. Acad. Sci. USA , 2011 . 108 ( 7 ): 2651 DOI: 10.1073/pnas.1015862108 http://doi.org/10.1073/pnas.1015862108 .

B.P. Lee , S. Konst . Adv. Mater. , 2014 . 26 ( 21 ): 3415 DOI: 10.1002/adma.v26.21 http://doi.org/10.1002/adma.v26.21 .

B.P. Lee , A. Narkar , R. Wilharm . Sens. Actuators B , 2016 . 227 ( 1 ): 248 http://www.sciencedirect.com/science/article/pii/S0925400514011757 http://www.sciencedirect.com/science/article/pii/S0925400514011757 , .

P. Glass , H. Chung , N.R. Washburn , M. Sitti . Langmuir , 2009 . 25 ( 12 ): 6607 DOI: 10.1021/la9009114 http://doi.org/10.1021/la9009114 .

B. Malisova , S. Tosatti , M. Textor , K. Gademann , S. Zürcher . Langmuir , 2010 . 26 ( 6 ): 4018 DOI: 10.1021/la903486z http://doi.org/10.1021/la903486z .

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