Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels

Jun-ying Weng; Zhuo Tang; Ying Guan; X.X. Zhu; Yong-jun Zhang

doi:10.1007/s10118-017-1962-1

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Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels

Papers | Updated：2021-02-18

- Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels
- Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels
- Chinese Journal of Polymer Science 2017年35卷第10期页码：1212-1221
- Affiliations：
  
  a.Key Laboratory of Functional Polymer Materials and State Key Laboratory of Medicinal Chemical Biology, The Co-Innovation Center of Chemistry and Chemical Engineering of Tianjin, Institute of Polymer Chemistry, College of Chemistry, Nankai University, Tianjin 300071, China
  b.Department of Chemistry, Université de Montréal, C. P. 6128, Succursale Centre-ville, Montreal, QC, H3C 3J7, Canada
- Author bio：
  
  Ying Guan (关英), E-mail:yingguan@nankai.edu.cn
  Yong-jun Zhang (张拥军), E-mail:yongjunzhang@nankai.edu.cn
- Funds：
  
  the National Natural Science Foundation of China(21374048);the National Natural Science Foundation of China(51625302);Tianjin Committee of Science and Technology(16JCZDJC32900);Supplementary material is available in the online version of this article at http://dx.doi.org/10.1007/s10118-017-1962-1.
- DOI：10.1007/s10118-017-1962-1
  中图分类号：
- 收稿：2017-03-16，
  
  修回：2017-4-13，
  
  录用：2017-4-17，
  
  纸质出版：2017-10-05
- Accepted：
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Jun-ying Weng, Zhuo Tang, Ying Guan, 等. Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels[J]. Chinese Journal of Polymer Science, 2017,35(10):1212-1221.

Jun-ying Weng, Zhuo Tang, Ying Guan, et al. Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels[J]. Chinese Journal of Polymer Science, 2017, 35(10): 1212-1221.
Jun-ying Weng, Zhuo Tang, Ying Guan, 等. Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels[J]. Chinese Journal of Polymer Science, 2017,35(10):1212-1221. DOI： 10.1007/s10118-017-1962-1.

Jun-ying Weng, Zhuo Tang, Ying Guan, et al. Assembly of Highly Ordered 2D Arrays of Silver-PNIPAM Hybrid Microgels[J]. Chinese Journal of Polymer Science, 2017, 35(10): 1212-1221. DOI： 10.1007/s10118-017-1962-1.

摘要

Abstract

A strategy was developed for the synthesis of highly ordered 2D arrays of Ag-PNIPAM hybrid microgel. The highly ordered 2D arrays of PNIPAM microgel were prepared by dispersing PNIPAM microgel on a charge-reversible substrate. The microgel spheres self-assembled into a 3D colloidal crystal

and the first 111 plane was fixed

in situ

onto the substrate as a result of spontaneous charge reversal of the substrate

leaving a high-quality 2D array of PNIPAM microgel. Ag nanoparticles were then synthesized

in situ

inside the microgel spheres by introduction of Ag

ions into the microgel spheres and reduction with sodium borohydride. The resulting 2D arrays are highly ordered. The inter-particle distance in the array can be tuned. In addition

the method allows the synthesis of large size arrays and the use of nonplanar substrate.

关键词

Keywords

references

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