Progress in Fluorene-based Wide-bandgap Steric Semiconductors

Meng-na Yu; Chang-jin Ou; Bin Liu; Dong-qing Lin; Yu-yu Liu; Wei Xue; Zong-qiong Lin; Jin-yi Lin; Yan Qian; Sha-sha Wang; Hong-tao Cao; Lin-yi Bian; Ling-hai Xie; Wei Huang

doi:10.1007/s10118-017-1897-6

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Progress in Fluorene-based Wide-bandgap Steric Semiconductors

Feature Article | Updated：2021-02-18

- Progress in Fluorene-based Wide-bandgap Steric Semiconductors
- Progress in Fluorene-based Wide-bandgap Steric Semiconductors
- Chinese Journal of Polymer Science 2017年35卷第2期页码：155-170
- Affiliations：
  
  a.Center for Molecular Systems and Organic Devices (CMSOD), Key Laboratory for Organic Electronics and Information Displays & Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing University of Posts & Telecommunications, Nanjing 210023, China
  b.Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (Nanjing Tech), Nanjing 211816, China
- Author bio：
  
  Ling-hai Xie (解令海), E-mail:iamlhxie@njupt.edu.cn
  Wei Huang (黄维), E-mail:iamwhuang@njupt.edu.cn
- Funds：
  
  the National Natural Science Funds for Excellent Young Scholar(21322402);the National Natural Science Foundation of China(21274064);the National Natural Science Foundation of China(61475074);the National Natural Science Foundation of China(21504041);the National Natural Science Foundation of China(61136003);University of Jiangsu Province Natural Science Foundation Project(14KJB510027);Natural Science Foundation of Jiangsu Province(BM2012010);Excellent Science and Technology Innovation Team of Jiangsu Higher Education Institutions, Synergetic Innovation Center for Organic Electronics and Information Displays, Natural Science of the Education Committee of Jiangsu Province(15KJB430019);Jiangsu Planned Projects for Postdoctoral Research Funds(1501019B)
- DOI：10.1007/s10118-017-1897-6
  中图分类号：
- 收稿：2016-10-05，
  
  修回：2016-11-10，
  
  录用：2016-11-16，
  
  纸质出版：2017-02
- Accepted：
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Meng-na Yu, Chang-jin Ou, Bin Liu, 等. Progress in Fluorene-based Wide-bandgap Steric Semiconductors[J]. Chinese Journal of Polymer Science, 2017,35(2):155-170.

Meng-na Yu, Chang-jin Ou, Bin Liu, et al. Progress in Fluorene-based Wide-bandgap Steric Semiconductors[J]. Chinese Journal of Polymer Science, 2017, 35(2): 155-170.
Meng-na Yu, Chang-jin Ou, Bin Liu, 等. Progress in Fluorene-based Wide-bandgap Steric Semiconductors[J]. Chinese Journal of Polymer Science, 2017,35(2):155-170. DOI： 10.1007/s10118-017-1897-6.

Meng-na Yu, Chang-jin Ou, Bin Liu, et al. Progress in Fluorene-based Wide-bandgap Steric Semiconductors[J]. Chinese Journal of Polymer Science, 2017, 35(2): 155-170. DOI： 10.1007/s10118-017-1897-6.

摘要

Abstract

Molecular bulks are favorable for the thermal and morphological stability in organic wide-bandgap semiconducting polymers with potential applications in both information and energy electronics. In this review

we present our progress in the design of fluorene-based bulky semiconductors with a fractal four-element pattern. Firstly

we established one-pot methods to spirofluorenes

especially spiro[fluorene-9

9'-xanthene] (SFX) serving as the next-generation spiro-based semiconductors. Secondly

we observed the supramolecular forces at the bulky groups and discovered the supramolecular steric hindrance (SSH) effect on poly

morphisms

nanocrystals as well as device performance. Thus

a synergistically molecular attractor-repulsor theory (SMART) was proposed for the control of nanocrystal morphology

thin film phase and morphology. Thirdly

the third possible type of defects has been identified to generate green band (g-band) emission in wide-bandgap semiconductors by the introduction of molecular strain design of cyclofluorene. Finally

the first bulky polydiarylfluorene with highly crystalline and

conformation was achieved by an attractor-repulsor design of tadpole-shape monomer

which offered an effective platform to fabricate stable wide-bandgap semiconducting devices. All the discoveries offer the solid basis to break through bottlenecks of organic/polymer wide-bandgap semiconductors by the improvements of overall performances.

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Keywords

references

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