Ejection Dynamics of Semiflexible Polymers out of a Nanochannel

Zhou Li-qin; Yu Wan-cheng; Chen Yu-hao; Luo Kai-fu

doi:10.1007/s10118-016-1842-0

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Ejection Dynamics of Semiflexible Polymers out of a Nanochannel

PAPERS | Updated：2021-05-12

- Ejection Dynamics of Semiflexible Polymers out of a Nanochannel
- Ejection Dynamics of Semiflexible Polymers out of a Nanochannel
- Chinese Journal of Polymer Science 2016年34卷第10期页码：1196-1207
- Affiliations：
  
  Chinese Academy of Sciences Key Laboratory of Soft Matter Chemistry, and Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei 230026, China
- Author bio：
  
  Wan-cheng Yu (昱万程), E-mail: ywcheng@ustc.edu.cn
  Yu-hao Chen (陈宇浩), E-mail: cyh204@mail.ustc.edu.cn
- Funds：
  
  the National Natural Science Foundation of China(21225421 and 21474099);the 973 Program of Ministry of Science and Technology of China (MOST)(2014CB845605);the Fundamental Research Funds for the Central Universities(WK2060200020);the China Postdoctoral Science Foundation(2015M581998)
- DOI：10.1007/s10118-016-1842-0
  中图分类号：
- 收稿：2016-03-29，
  
  修回：2016-4-14，
  
  录用：2016-4-15，
  
  纸质出版：2016-10-05
- Accepted：
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Zhou Li-qin, Yu Wan-cheng, Chen Yu-hao, 等. Ejection Dynamics of Semiflexible Polymers out of a Nanochannel[J]. Chinese Journal of Polymer Science, 2016,34(10):1196-1207.

Zhou Li-qin, Yu Wan-cheng, Chen Yu-hao, et al. Ejection Dynamics of Semiflexible Polymers out of a Nanochannel[J]. Chinese Journal of Polymer Science, 2016, 34(10): 1196-1207.
Zhou Li-qin, Yu Wan-cheng, Chen Yu-hao, 等. Ejection Dynamics of Semiflexible Polymers out of a Nanochannel[J]. Chinese Journal of Polymer Science, 2016,34(10):1196-1207. DOI： 10.1007/s10118-016-1842-0.

Zhou Li-qin, Yu Wan-cheng, Chen Yu-hao, et al. Ejection Dynamics of Semiflexible Polymers out of a Nanochannel[J]. Chinese Journal of Polymer Science, 2016, 34(10): 1196-1207. DOI： 10.1007/s10118-016-1842-0.

摘要

Abstract

Using theoretical analysis and three-dimensional Langevin dynamics simulations

we investigate the influence of chain rigidity on the ejection dynamics of polymers from a nanochannel. We find that there exist two distinct dynamical regimes divided by a critical chain length for both flexible and semiflexible chains. At the short chain regime

semiflexible chains eject faster than flexible chains of the same chain length due to the longer occupying length. In contrast

at the long chain regime

semiflexible chains eject slower than flexible ones as the effective entropic driving force decreases. Based on these results

we propose that the nanochannels could be used to separate flexible and semiflexible chains effectively

关键词

Keywords

references

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