Fluorinated <italic style="font-style: italic">p</italic>-<italic style="font-style: italic">n</italic> Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device

Liu Bin; Bao Yan; Ling Hai-feng; Zhu Wen-sai; Gong Rui-jun; Lin Jin-yi; Xie Ling-hai; Yi Ming-dong; Huang Wei

doi:10.1007/s10118-016-1826-0

Your Location：

Home >

Browse articles >

Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device

PAPERS | Updated：2021-05-12

- Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device
- Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device
- Chinese Journal of Polymer Science 2016年34卷第10期页码：1183-1195
- Affiliations：
  
  a Centre for Molecular Systems and Organic Devices, Key Laboratory for Organic Electronics and Information Displays & Institute of Advanced Materials, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing University of Posts & Telecommunications, Nanjing 210023, China
  b Key Laboratory of Flexible Electronics & Institute of Advanced Materials, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University, Nanjing 211816, China
- Author bio：
  
  Ling-hai Xie (解令海), E-mail: iamlhxie@njupt.edu.cn
  Ming-dong Yi (仪明东), E-mail: iammdyi@njupt.edu.cn
  Wei Huang (黄维), E-mail: iamwhuang@njupt.edu.cn
- Funds：
  
  the National Natural Science Funds for Excellent Young Scholar(21322402);the National Natural Science Foundation of China(21274064, 61475074, 21504041 and 61136003);University of Jiangsu Province Natural Science Foundation Project(14KJB510027);Natural Science Foundation of Jiangsu Province(BM2012010);Synergetic Innovation Center for Organic Electronics and Information Displays, Natural Science of the Education Committee of Jiangsu Province(15KJB430019);Jiangsu Planned Projects for Postdoctoral Research Funds(1501019B)
- DOI：10.1007/s10118-016-1826-0
  中图分类号：
- 收稿：2016-03-21，
  
  修回：2016-4-28，
  
  录用：2016-5-1，
  
  纸质出版：2016-10-05
- Accepted：
Scan QR Code
Liu Bin, Bao Yan, Ling Hai-feng, 等. Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device[J]. Chinese Journal of Polymer Science, 2016,34(10):1183-1195. DOI: 10.1007/s10118-016-1826-0.

Liu Bin, Bao Yan, Ling Hai-feng, et al. Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device[J]. Chinese Journal of Polymer Science, 2016, 34(10): 1183-1195. DOI: 10.1007/s10118-016-1826-0.
Liu Bin, Bao Yan, Ling Hai-feng, 等. Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device[J]. Chinese Journal of Polymer Science, 2016,34(10):1183-1195. DOI: 10.1007/s10118-016-1826-0. DOI：

Liu Bin, Bao Yan, Ling Hai-feng, et al. Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device[J]. Chinese Journal of Polymer Science, 2016, 34(10): 1183-1195. DOI: 10.1007/s10118-016-1826-0. DOI：

摘要

Abstract

In this study

a kind of fluorinated copolyfluorene

named poly[(4-(octyloxy)-9

9-diphenylfluorene-2

7-diyl)-

alt

-(2

6-tetrafluoro-1

4-phenylene)] (PODPF-TFP)

is synthesized by facile palladium-based direct aromatization. Compared to the non-fluorinated counterpart

poly[(4-(octyloxy)-9

9-diphenylfluorene-2

7-diyl)-

alt

-phenylene)] (PODPF-P)

deeper HOMO/LUMO energy level combined with steric hindrance effect endow PODPF-TFP with excellent spectra and morphology stability. Finally

organic field-effect transistor (OFET) memory devices are fabricated with PODPF-P/PODPF-TFP as the dielectric layers

and they both exhibit flash type storage characteristic. Owing to the electronegativity of fluorine atom

the device based on PODPF-TFP exhibits larger memory window and more stable I

off

ratio during a retention time of 10

s as well as a better aging stability. The present study suggests that fluorinated

p-n

copolyfluorene electrets could enhance the capabilities of charge trapping and storage

which are promising for OFET memory devices.

关键词

Keywords

references

L.H. Xie, , C.R. Yin, , W.Y. Lai, . . Fan, Q.L, Huang, W.Prog. Polym. Sci. , 2012 . 37 1192 DOI: 10.1016/j.progpolymsci.2012.02.003 http://doi.org/10.1016/j.progpolymsci.2012.02.003 .

Ling, Q.D., Liaw, D.J., Zhu, C.X., Chan, D.S.H., Kang, E.T. and Neoh, K.G., Prog. Polym. Sci., 2008, 33: 917

Y.C. Yang, , F. Pan, , Q. Liu, . . Liu, M, Zeng, F.Nano Lett. , 2009 . 9 1636 .

Gao, S., Song, C., Chen, C., Zeng, F. and Pan, F., J. Phys. Chem. C, 2012, 116: 17955

S. Nau, . . Sax, S, List-Kratochvil, E.J.W.Adv. Mater. , 2014 . 26 2508 .

Sekitani, T., Yokota, T., Zschieschang, U., Klauk, H., Bauer, S., Takeuchi, K., Takamiya, M., Sakurai, T. and Someya, T., Science, 2009, 326: 1516

L. Zhang, , T. Wu, , Y.L. Guo, , Y. Zhao, , X.N. Sun, , Y.G. Wen, . . Yu, G, Liu, Y.Q.Sci. Rep. , 2013 . 3 1080 .

Kim, S.J. and Lee, J.S., Nano Lett., 2010, 10: 2884

S. Park, , G. Wang, , B. Cho, , Y. Kim, , S. Song, , Y. Ji, . . Yoon, M.H, Lee, T.Nature Nanotechnol. , 2012 . 7 438 DOI: 10.1038/nnano.2012.81 http://doi.org/10.1038/nnano.2012.81 .

Yu, W.L., Meng, H., Pei, J. and Huang, W., J. Am. Chem. Soc., 1998, 120: 11808

W.L. Yu, , H. Meng, , J. Pei, , W. Huang, . . Li, Y.F, Heeger, A.J.Macromolecules , 1998 . 31 4838 DOI: 10.1021/ma9800212 http://doi.org/10.1021/ma9800212 .

Robinson, L., Isaksson, J., Robinson, N.D. and Berggren, M., Surf. Sci., 2006, 600: 148

H.H. Fong, , J.K. Lee, , Y.F. Lim, , A.A. Zakhidov, , W.W.H. Wong, , A.B. Holmes, . . Ober, C.K, Malliaras, G.G.Adv. Mater. , 2011 . 23 735 .

Deng, J.N., Wang, W.B., Zheng, Z.H., Ding, X.B. and Peng, Y.X., Chinese J. Polym. Sci., 2014, 32(7): 817

M.G Dhara, , S. Banerjee, . . Prog. Polym. Sci. , 2010 . 35 1022 DOI: 10.1016/j.progpolymsci.2010.04.003 http://doi.org/10.1016/j.progpolymsci.2010.04.003 .

N. Marjanovic, , T.B. Singh, , G. Dennler, , S. Gunes, , H. Neugebauer, , N.S. Sariciftci, , R Schwodiauer, , S. Bauer, . . Org. Electron. , 2006 . 7 188 DOI: 10.1016/j.orgel.2006.01.002 http://doi.org/10.1016/j.orgel.2006.01.002 .

Y.F. Li, . . Accounts Chem. Res. , 2012 . 45 723 DOI: 10.1021/ar2002446 http://doi.org/10.1021/ar2002446 .

S. Nau, , C. Wolf, , S Sax, , E.J.W. List-Kratochvil, . . Adv. Mater. , 2015 . 27 1048 DOI: 10.1002/adma.201403295 http://doi.org/10.1002/adma.201403295 .

C.C. Shih, , Y.C. Chiu, , W.Y. Lee, , J.Y Chen, , W.C. Chen, . . Adv. Funct. Mater. , 2015 . 25 1511 DOI: 10.1002/adfm.v25.10 http://doi.org/10.1002/adfm.v25.10 .

Y.H. Chou, , H.C. Chang, , C.L Liu, , W.C. Chen, . . Polym. Chem. , 2015 . 6 341 DOI: 10.1039/C4PY01213E http://doi.org/10.1039/C4PY01213E .

Y.C. Chiu, , C.L. Liu, , W.Y. Lee, , Y.G. Chen, , T Kakuchi, , W.C. Chen, . . Npg Asia Mater. , 2013 . 5 .

H.S. Sun, , Y.C. Chiu, , W.Y. Lee, , Y.G. Chen, , A. Hirao, , T. Satoh, , T Kakuchi, , W.C. Chen, . . Macromolecules , 2015 . 48 3907 DOI: 10.1021/acs.macromol.5b00651 http://doi.org/10.1021/acs.macromol.5b00651 .

K.J. Baeg, , Y.Y. Noh, , J. Ghim, , B Lim, , D.Y. Kim, . . Adv. Funct. Mater. , 2008 . 18 3678 DOI: 10.1002/adfm.v18:22 http://doi.org/10.1002/adfm.v18:22 .

W. Huang, , H. Meng, , W.L. Yu, , J. Pei, , Z.K Chen, , Y.H. Lai, . . Macromolecules , 1999 . 32 118 DOI: 10.1021/ma9813237 http://doi.org/10.1021/ma9813237 .

H. Meng, , Z.K Chen, , W. Huang, . . J. Phys. Chem. B , 1999 . 103 6429 .

A.J. Heeger, . . Chem. Soc. Rev. , 2010 . 39 2354 DOI: 10.1039/b914956m http://doi.org/10.1039/b914956m .

A. Facchetti, , M.H. Yoon, , C.L. Stern, , H.E Katz, , T.J. Marks, . . Angew. Chem. Int. Ed. , 2003 . 42 3900 DOI: 10.1002/(ISSN)1521-3773 http://doi.org/10.1002/(ISSN)1521-3773 .

Y.Y. Liang, , D.Q. Feng, , Y. Wu, , S.T. Tsai, , G. Li, , C Ray, , L.P. Yu, . . J. Am. Chem. Soc. , 2009 . 131 7792 DOI: 10.1021/ja901545q http://doi.org/10.1021/ja901545q .

X.F. Liu, , B.B.Y. Hsu, , Y.M. Sun, , C.K. Mai, , A.J Heeger, , G.C. Bazan, . . J. Am. Chem. Soc. , 2014 . 136 16144 DOI: 10.1021/ja510088x http://doi.org/10.1021/ja510088x .

H.J. Son, , W. Wang, , T. Xu, , Y.Y. Liang, , Y.E. Wu, , G Li, , L.P. Yu, . . J. Am. Chem. Soc. , 2011 . 133 1885 DOI: 10.1021/ja108601g http://doi.org/10.1021/ja108601g .

Y.H. Chou, , N.H. You, , T. Kurosawa, , W.Y. Lee, , T. Higashihara, , M Ueda, , W.C. Chen, . . Macromolecules , 2012 . 45 6946 DOI: 10.1021/ma301326r http://doi.org/10.1021/ma301326r .

A.D. Yu, , W.Y. Tung, , Y.C. Chiu, , C.C. Chueh, , G.S Liou, , W.C. Chen, . . Macromol. Rapid Commun. , 2014 . 35 1039 DOI: 10.1002/marc.201400089 http://doi.org/10.1002/marc.201400089 .

L.H. Xie, , X.Y. Hou, , Y.R. Hua, , C. Tang, , F. Liu, , Q.L Fan, , W. Huang, . . Org. Lett. , 2006 . 8 3701 DOI: 10.1021/ol061268j http://doi.org/10.1021/ol061268j .

L.H. Xie, , T. Fu, , X.Y. Hou, , C. Tang, , Y.R. Hua, , R.J. Wang, , Q.L. Fan, , B. Peng, , W Wei, , W. Huang, . . Tetrahedron Lett. , 2006 . 47 6421 DOI: 10.1016/j.tetlet.2006.06.143 http://doi.org/10.1016/j.tetlet.2006.06.143 .

L.H. Xie, , X.Y. Hou, , C. Tang, , Y.R. Hua, , R.J. Wang, , R.F. Chen, , Q.L. Fan, , L.H. Wang, , W. Wei, , B Peng, , W. Huang, . . Org. Lett. , 2006 . 8 1363 DOI: 10.1021/ol060109x http://doi.org/10.1021/ol060109x .

L.H. Xie, , Q.D. Ling, , X.Y Hou, , W. Huang, . . J. Am. Chem. Soc. , 2008 . 130 2120 DOI: 10.1021/ja076720o http://doi.org/10.1021/ja076720o .

C.R. Yin, , Y. Han, , L. Li, , S.H. Ye, , W.W. Mao, , M.D. Yi, , H.F. Ling, , L.H. Xie, , G.W Zhang, , W. Huang, . . Polym. Chem. , 2013 . 4 2540 DOI: 10.1039/c3py21154a http://doi.org/10.1039/c3py21154a .

Z.D. Liu, , Y.Z. Chang, , C.J. Ou, , J.Y. Lin, , L.H. Xie, , C.R. Yin, , M.D. Yi, , Y. Qian, , N.E Shi, , W. Huang, . . Polym. Chem. , 2011 . 2 2179 DOI: 10.1039/c1py00203a http://doi.org/10.1039/c1py00203a .

J.Y. Lin, , W. Li, , Z.Z. Yu, , M.D. Yi, , H.F. Ling, , L.H. Xie, , S.B Li, , W. Huang, . . J. Mater. Chem. C , 2014 . 2 3738 DOI: 10.1039/c3tc32441a http://doi.org/10.1039/c3tc32441a .

M.M. Sun, , W. Wang, , L.Y. Liang, , S.H. Yan, , M.L Zhou, , Q.D. Ling, . . Chinese J. Polym. Sci. , 2015 . 33 ( 5 ): 783 DOI: 10.1007/s10118-015-1555-9 http://doi.org/10.1007/s10118-015-1555-9 .

J.Y. Lin, , W.S. Zhu, , F. Liu, , L.H. Xie, , L. Zhang, , R. Xia, , G.C Xing, , W. Huang, . . Macromolecules , 2014 . 47 1001 DOI: 10.1021/ma402585n http://doi.org/10.1021/ma402585n .

W. Lu, , J. Kuwabara, , T. Iijima, , H. Higashimura, , H Hayashi, , T. Kanbara, . . Macromolecules , 2012 . 45 4128 DOI: 10.1021/ma3004899 http://doi.org/10.1021/ma3004899 .

M. Wakioka, , Y Kitano, , F. Ozawa, . . Macromolecules , 2013 . 46 370 DOI: 10.1021/ma302558z http://doi.org/10.1021/ma302558z .

B. Liu, , J. Lin, , Z. Lei, , M. Sun, , L. Xie, , W. Xue, , C. Yin, , X Zhang, , W. Huang, . . Macromol. Chem. Phys. , 2015 . 216 1043 DOI: 10.1002/macp.v216.10 http://doi.org/10.1002/macp.v216.10 .

M.F. Liu, , Y.L. Chen, , C Zhang, , Z.S. Bo, . . Chinese J. Polym. Sci. , 2012 . 30 ( 2 ): 308 DOI: 10.1007/s10118-012-1127-1 http://doi.org/10.1007/s10118-012-1127-1 .

X.N. Sun, , Y.Q. Liu, , C.A. Di, , Y.G. Wen, , Y.L. Guo, , L. Zhang, , Y Zhao, , G. Yu, . . Adv. Mater. , 2011 . 23 1009 DOI: 10.1002/adma.v23.8 http://doi.org/10.1002/adma.v23.8 .

A. Calzolari, , B. Vercelli, , A. Ruini, , T Virgili, , M. Pasini, . . J. Phys. Chem. C , 2013 . 117 26760 DOI: 10.1021/jp409996m http://doi.org/10.1021/jp409996m .

浏览量

Downloads

CSCD

文章被引用时，请邮件提醒。

Submit

工具集

关联资源

A Facile Photo-cross-linking Method for Polymer Gate Dielectrics and Their Applications in Fully Solution Processed Low Voltage Organic Field-effect Transistors on Plastic Substrate

Squaramide-directed Cooperative One-dimensional Assembly in Telechelic Polydimethylsiloxane for Hierarchical Network Formation

Circularly Polarized Luminescence Based on Helical Polymers: Structure-Property Relationships and Regulation Mechanisms

Energy Storage Performance of Supercapacitors with Polyelectrolyte Surface Coatings: Effects of Dielectric Contrast

Sequence-encoded Conformation Pathways in Viscoelastic Microphase Separation of Multiblock Copolymers

Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device

Fluorinated p-n Type Copolyfluorene as Polymer Electret for Stable Nonvolatile Organic Transistor Memory Device

DOI：10.1007/s10118-016-1826-0

摘要

Abstract

关键词

Keywords

references