Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes

Jian-hua Li; Shuang-shuang Wang; De-bin Zhang; Xing-xing Ni; Qi-qing Zhang

doi:10.1007/s10118-016-1808-2

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Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes

PAPERS | Updated：2021-05-12

- Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes
- Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes
- Chinese Journal of Polymer Science 2016年34卷第7期页码：805-819
- Affiliations：
  
  Institute of Biomedical and Pharmaceutical Technology, Fuzhou University, Fuzhou 350001, China
- Author bio：
  
  Jian-hua Li (李建华), E-mail: jhli_2005@163.com
  Qi-qing Zhang (张其清), E-mail: zhangqiq@126.com
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (No. 51303028) and Test Center of Fuzhou University.
- DOI：10.1007/s10118-016-1808-2
  中图分类号：
- 收稿：2015-12-16，
  
  修回：2016-3-9，
  
  录用：2016-3-18，
  
  纸质出版：2016-07
- Accepted：
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Jian-hua Li, Shuang-shuang Wang, De-bin Zhang, 等. Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes[J]. Chinese Journal of Polymer Science, 2016,34(7):805-819.

Jian-hua Li, Shuang-shuang Wang, De-bin Zhang, et al. Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes[J]. Chinese Journal of Polymer Science, 2016, 34(7): 805-819.
Jian-hua Li, Shuang-shuang Wang, De-bin Zhang, 等. Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes[J]. Chinese Journal of Polymer Science, 2016,34(7):805-819. DOI： 10.1007/s10118-016-1808-2.

Jian-hua Li, Shuang-shuang Wang, De-bin Zhang, et al. Amino Acids Functionalized Graphene Oxide for Enhanced Hydrophilicity and Antifouling Property of Poly(vinylidene fluoride) Membranes[J]. Chinese Journal of Polymer Science, 2016, 34(7): 805-819. DOI： 10.1007/s10118-016-1808-2.

摘要

Abstract

Herein

functionalized graphene oxide (GO) was prepared by the covalent functionalization with amino acids (lysine

glycine

glutamic acid and tyrosine) in this study. Zeta potential results demonstrated that covalent functionalization of GO with amino acids was favourable for their homogeneous dispersion in water and organic solvents. Based on the higher absolute value of zeta potential and the better dipersion stability of GO-lysine

the PVDF/GO-lysine hybrid membranes were then prepared

via

the phase inversion induced by immersion precipitation technique. SEM images showed a better pore diameter and porosity distribution on the PVDF/GO-lysine membrane surface. The zeta potential absolute value of the PVDF/GO-lysine membrane surface was higher than that of the virgin PVDF membrane. Furthermore

the PVDF/GO-lysine membranes surface exhibited good hydrophilicity. The water flux of PVDF/GO-lysine membranes can reach two times of that of the virgin PVDF membrane. And the BSA adsorbed amount on PVDF/GO-lysine surface was decreased to 0.82 mg/cm

for PVDF/GO-lysine-8% membrane. Filtration experiment results indicated that the fouling resistance was significantly improved for the PVDF/GO-lysine membranes. As a result

lysine functionalized GO will provide a promising method to fabricate graphene oxide based hybrid membranes with effective antifouling property and hydrophilicity.

关键词

Keywords

references

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