Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water

Hua-ji Liu; Yue-yue Xu; Yu Chen

doi:10.1007/s10118-016-1779-3

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Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water

PAPERS | Updated：2021-05-12

- Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water
- Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water
- Chinese Journal of Polymer Science 2016年34卷第5期页码：585-593
- Affiliations：
  
  Department of Chemistry, School of Sciences, Tianjin University, and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin), Tianjin 300354, China
- Author bio：
  
  Yu Chen (陈宇), E-mail: chenyu@tju.edu.cn
- Funds：
  
  the National Natural Science Foundation of China(20804027);the National Natural Science Foundation of China(21274106)
- DOI：10.1007/s10118-016-1779-3
  中图分类号：
- 收稿：2015-11-10，
  
  修回：2016-1-3，
  
  录用：2016-1-3，
  
  纸质出版：2016-05
- Accepted：
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Hua-ji Liu, Yue-yue Xu, Yu Chen. Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water[J]. Chinese Journal of Polymer Science, 2016,34(5):585-593.

Hua-ji Liu, Yue-yue Xu, Yu Chen. Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water[J]. Chinese Journal of Polymer Science, 2016, 34(5): 585-593.
Hua-ji Liu, Yue-yue Xu, Yu Chen. Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water[J]. Chinese Journal of Polymer Science, 2016,34(5):585-593. DOI： 10.1007/s10118-016-1779-3.

Hua-ji Liu, Yue-yue Xu, Yu Chen. Influence of Sodium Dodecyl Sulfate on the Phase Transition of Thermoresponsive Hyperbranched Polymer in Water[J]. Chinese Journal of Polymer Science, 2016, 34(5): 585-593. DOI： 10.1007/s10118-016-1779-3.

摘要

Abstract

The influence of sodium dodecyl sulfate (SDS) on the cloud point temperature (

) of the aqueous solution of thermoresponsive hyperbranched polyethylenimine derivative HPEI-IBAm was studied systematically. When pH was below 8.5

HPEI-IBAm was positively-charged. Initially

the

of HPEI-IBAm decreased significantly

followed by an obvious increase with the increase of SDS concentration. The lower the pH was

the higher the SDS concentration was required to achieve the minimum

. When pH was above 8.5

HPEI-IBAm was neutral and raising the SDS concentration led to the gradual increase of

. Compared to linear poly(

-isopropyl acrylamide) (PNIPAm)

the

of the current hyperbranched HPEI-IBAm was more sensitive to SDS. The thermoresponsive HPEI-IBAm/SDS complex was used as host to accommodate the non-polar pyrene in water. The lowest SDS concentration for effectively enhancing the solubility of pyrene in water was around 6.4 mmol·L

-1

. When HPEI-IBAm was present

the SDS concentration threshhold was decreased to about 0.31 mmol·L

-1

. Fluorescence technique with pyrene as the hydrophobic probe demonstrated that the SDS concentration of 7.2 mmol·L

-1

was required to form the hydrophobic domain to accommodate pyrene guests without HPEI-IBAm

while only 0.2 mmol·L

-1

of SDS was required in the presence of HPEI-IBAm.

关键词

Keywords

references

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