Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings

Kai-qiang Zhang; Jing-zhe Cai; Xiao-hui Li; Hui Li; Yun-hui Zhao; Xiao-yan Yuan

doi:10.1007/s10118-015-1563-9

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Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings

PAPER | Updated：2021-06-21

- Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings
- Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings
- Chinese Journal of Polymer Science 2015年33卷第1期页码：153-162
- Affiliations：
  
  a.School of Materials Science and Engineering, and Tianjin Key Laboratory of Composite and Functional Materials, Tianjin University, Tianjin 300072, China
  b.School of Chemistry and Chemical Engineering, Shandong Key Laboratory of Fluorine Chemistry and Chemical Engineering Materials, University of Jinan, Jinan 250022, China
- Author bio：
  
  †Kai-qiang Zhang and Jing-zhe Cai contributed equally to this work.
  **Yun-hui Zhao (赵蕴慧), E-mail: zhaoyunhui@tju.edu.cn
  Xiao-yan Yuan (袁晓燕), E-mail: yuanxy@tju.edu.cn
- Funds：
  
  National Natural Science Foundation of China(51273146;51103061);Natural Science Foundation of Tianjin, China(14ZCZDGX00008)
- DOI：10.1007/s10118-015-1563-9
  中图分类号：
- 收稿：2014-05-30，
  
  修回：2014-06-18，
  
  录用：2014-07-15，
  
  纸质出版：2015-01
- Accepted：
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Kai-qiang Zhang, Jing-zhe Cai, Xiao-hui Li, 等. Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings[J]. Chinese Journal of Polymer Science, 2015,33(1):153-162.

Kai-qiang Zhang, Jing-zhe Cai, Xiao-hui Li, et al. Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings[J]. Chinese Journal of Polymer Science, 2015, 33(1): 153-162.
Kai-qiang Zhang, Jing-zhe Cai, Xiao-hui Li, 等. Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings[J]. Chinese Journal of Polymer Science, 2015,33(1):153-162. DOI： 10.1007/s10118-015-1563-9.

Kai-qiang Zhang, Jing-zhe Cai, Xiao-hui Li, et al. Balance of Polyacrylate-Fluorosilicone Block Copolymers as Icephobic Coatings[J]. Chinese Journal of Polymer Science, 2015, 33(1): 153-162. DOI： 10.1007/s10118-015-1563-9.

摘要

Abstract

Polyacrylate-fluorosilicone block copolymers

namely

polyacrylate-

-polydimethylsiloxane and polyacrylate-

-polymethyltrifluoropropylsiloxane were synthesized for fabricating icephobic coatings. The surface morphology and chemical composition of the block copolymers were characterized by atomic force microscopy and X-ray photoelectron spectroscopy

suggesting that the fluorosilicone blocks aggregated on the top of the copolymer surfaces. Results of water contact angles and ice shear strength demonstrated a certain amount adding of methacryloisobutyl polyhedral oligomeric silsesquioxane could lead to the decrease of contact angle hysteresis and increase of surface roughness

consequently resulting in significant reduction of the ice adhesion strength. Therefore

the block copolymers with the combined advantages of silicone and fluoropolymers could be potentially applied as icephobic coatings.

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