SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE

Guo-xin Jiang; Chun-lei Bian; Jun-qiao Ding; Li-xiang Wang

doi:10.1007/s10118-013-1279-7

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SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE

Special Issue: In Honor of the 80th Birthday of Professor Fosong Wang (Part I) | Updated：2023-01-03

- SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE
- SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE
- Chinese Journal of Polymer Science 2013年31卷第5期页码：787-797
- Affiliations：
  
  a.State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China
  b.University of the Chinese Academy of Sciences, Beijing 100049, China
- Author bio：
  
  **Jun-qiao Ding (丁军侨), E-mail: junqiaod@ciac.jl.cn
  Li-xiang Wang (王利祥), E-mail: lixiang@ciac.jl.cn
- Funds：
  
  973 Project(2009CB623601;2009CB930603);National Natural Science Foundation of China(21074130);Science Fund for Creative Research Groups(20921061)
- DOI：10.1007/s10118-013-1279-7
  中图分类号：
- 收稿：2012-12-19，
  
  修回：2013-01-25，
  
  录用：2013-02-04，
  
  纸质出版：2013-05
- Accepted：
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Guo-xin Jiang, Chun-lei Bian, Jun-qiao Ding, 等. SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE[J]. Chinese Journal of Polymer Science, 2013,31(5):787-797.

Guo-xin Jiang, Chun-lei Bian, Jun-qiao Ding, et al. SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE[J]. Chinese Journal of Polymer Science, 2013, 31(5): 787-797.
Guo-xin Jiang, Chun-lei Bian, Jun-qiao Ding, 等. SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE[J]. Chinese Journal of Polymer Science, 2013,31(5):787-797. DOI： 10.1007/s10118-013-1279-7.

Guo-xin Jiang, Chun-lei Bian, Jun-qiao Ding, et al. SYNTHESIS AND CHARACTERIZATION OF BLUE LIGHT-EMITTING POLY(ARYL ETHER)S CONTAINING PYRIMIDINE-INCORPORATED OLIGOFLUORENE PENDANTS WITH BIPOLAR FEATURE[J]. Chinese Journal of Polymer Science, 2013, 31(5): 787-797. DOI： 10.1007/s10118-013-1279-7.

摘要

Abstract

Novel blue light-emitting poly(aryl ether)s comprising of bipolar oligofluorene pendants as chromophores have been designed and synthesized

in which pyrimidine and arylamine moieties are utilized as the electron acceptor and electron donor

respectively. Through varying π bridge length from monofluorene to bifluorene and end-cappers from hydrogen to carbazole and diphenylamine

the emission color of the resulting polymers covers from deep blue to greenish blue

and their HOMO and LUMO levels can be modulated to facilitate charge injection to improve the device performance. Polymer lightemitting diodes (PLEDs) are fabricated with the device structure of ITO/poly(3

4-ethylenedioxythiophene):poly(styrene sulfonic acid) (PEDOT:PSS) (50 nm)/polymer (80 nm)/Ca (10 nm)/Al (200 nm). Among these polymers

P2Cz5F-Py with bifluorene bridge and carbazole end-capper shows excellent trade-off between the efficiency and emission wavelength

having a peak luminous efficiency as high as 1.26 cd/A and Commission Internationale de L’Eclairage (CIE) coordinates of (0.17

0.17).

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