Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@<italic style="font-style: italic">f</italic>-CNTs Networks <italic style="font-style: italic">via</italic> Self-sacrificing Template Method

Shuang-Shuang Wang; Dian-Ying Feng; Zhi-Ming Zhang; Xia Liu; Kun-Peng Ruan; Yong-Qiang Guo; Jun-Wei Gu

doi:10.1007/s10118-024-3098-4

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Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method

RESEARCH ARTICLE | Updated：2024-06-26

- Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method
  Enhanced Publication
- Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method
- 高分子科学（英文版） 2024年42卷第7期页码：897-906
- Affiliations：
  
  a.Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, China
  b.Shandong Institute of Nonmetallic Materials, Jinan 250031, China
  c.Queen Mary University of London Engineering School, Northwestern Polytechnical University, Xi’an 710072, China
- Author bio：
  
  gyqnpu@163.com
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (No. 51973173), Technological Base Scientific Research Projects (Highly Thermally Conductive Nonmetal Materials), Natural Science Foundation of Chongqing, China (No. 2023NSCQ-MSX2547), Shaanxi Province Key Research and Development Plan Project (No. 2023-YBGY-461) and Fundamental Research Funds for the Central Universities, the Innovation Capability Support Program of Shaanxi (No. 2024RS-CXTD-57). This work was also financially supported by Polymer Electromagnetic Functional Materials Innovation Team of Shaanxi Sanqin Scholars. We would like to thank the Analytical & Testing Center of Northwestern Polytechnical University for XRD and others tests.;Electronic supplementary information (ESI) is available free of charge in the online version of this article at http://doi.org/10.1007/s10118-024-3098-4.
- DOI：10.1007/s10118-024-3098-4
  中图分类号：
- 纸质出版日期：2024-07-01，
  
  网络出版日期：2024-02-23，
  
  收稿日期：2023-11-30，
  
  修回日期：2023-01-09，
  
  录用日期：2024-01-19
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Wang, S. S.; Feng, D. Y.; Zhang, Z. M.; Liu, X.; Ruan, K. P.; Guo, Y. Q.; Gu, J. W. Highly thermally conductive polydimethylsiloxane composites with controllable 3D GO@f-CNTs networks via self-sacrificing template method. Chinese J. Polym. Sci. 2024, 42, 897–906

Shuang-Shuang Wang, Dian-Ying Feng, Zhi-Ming Zhang, et al. Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method[J]. Chinese Journal of Polymer Science, 2024,42(7):897-906.
Wang, S. S.; Feng, D. Y.; Zhang, Z. M.; Liu, X.; Ruan, K. P.; Guo, Y. Q.; Gu, J. W. Highly thermally conductive polydimethylsiloxane composites with controllable 3D GO@f-CNTs networks via self-sacrificing template method. Chinese J. Polym. Sci. 2024, 42, 897–906 DOI： 10.1007/s10118-024-3098-4.

Shuang-Shuang Wang, Dian-Ying Feng, Zhi-Ming Zhang, et al. Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method[J]. Chinese Journal of Polymer Science, 2024,42(7):897-906. DOI： 10.1007/s10118-024-3098-4.

摘要

Hetero-structured GO@f-CNTs fillers prepared via chemical grafting method are constructed into controllable 3D GO@f-CNTs thermal conduction networks via self-sacrificing template method based on oxalic acid. When the size of oxalic acid is 0.24 mm and the volume fraction of GO@f-CNTs is 60 vol%

GO@f-CNTs/PDMS composites have optimal thermal conductivity (4.00 W/(m·K)).

Abstract

Constructing controllable thermal conduction networks is the key to efficiently improve thermal conductivities of polymer composites. In this work

graphite oxide (GO) and functionalized carbon nanotubes (

-CNTs) are combined to prepare “Line-Plane”-like hetero-structured thermally conductive GO@

-CNTs fillers

which are then performed to construct controllable 3D GO@

-CNTs thermal conduction networks

via

self-sacrificing template method based on oxalic acid. Subsequently

thermally conductive GO@

-CNTs/polydimethylsiloxane (PDMS) composites are fabricated

via

casting method. When the size of oxalic acid is 0.24 mm and the volume fraction of GO@

-CNTs is 60 vol%

GO@

-CNTs/PDMS composites present the optimal thermal conductivity coefficient (

4.00 W·m

−1

·K

−1

)

about 20 times that of the

of neat PDMS (0.20 W·m

−1

·K

−1

)

also much higher than the

(2.44 W·m

−1

·K

−1

) of GO/

-CNTs/PDMS composites with the same amount of randomly dispersed fillers. Meanwhile

the obtained GO@

-CNTs/PDMS composites have excellent thermal stability

whose

deviation is only about 3% after 500 thermal cycles (20−200 °C).

关键词

Keywords

PolydimethylsiloxaneHetero-structured thermally conductive fillersSelf-sacrificing templateThermal conduction networks

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Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method

Highly Thermally Conductive Polydimethylsiloxane Composites with Controllable 3D GO@f-CNTs Networks via Self-sacrificing Template Method

DOI：10.1007/s10118-024-3098-4

摘要

Abstract

关键词

Keywords

references