Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors

Yi-Fan Li; Yun-Long Guo; Yun-Qi Liu

doi:10.1007/s10118-023-2952-0

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Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors

REVIEW | Updated：2023-04-21

- Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors
- Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors
- 高分子科学（英文版） 2023年41卷第5期页码：652-670
- Affiliations：
  
  a.Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
  b.University of Chinese Academy of Sciences, Beijing 100049, China
- Author bio：
  
  guoyunlong@iccas.ac.cn(Y.L.G.)
  liuyq@iccas.ac.cn(Y.Q.L.)
- Funds：
  
  This work was financially supported by the National Key R&D Program of ‘Key Scientific Issues of Transformative Technology’ (No. 2018YFA0703200), the National Natural Science Foundation of China (Nos. U22A6002, 91833306, 21922511 and 51873216), the Strategic Priority Research Program of the Chinese Academy of Sciences (No. XDB30000000), the CAS Project for Young Scientists in Basic Research (No. YSBR-053), the CAS-Croucher Funding Scheme for Joint Laboratories, the CAS Cooperation Project (No. 121111KYSB20200036), and the Lu Jiaxi international team (No. GJTD-2020-02).;Yun-Long Guoreceived his Ph.D. degree in physical chemistry from the Institute of Chemistry, Chinese Academy of Sciences (ICCAS) in 2010. Now, he is a professor at ICCAS. His research interests include organic–inorganic hybrid perovskite electronics and functional organic field-effect transistors.Yun-Qi Liuis a professor at the Institute of Chemistry, Chinese Academy of Sciences (ICCAS). He graduated from Nanjing University in 1975 and received his Ph.D. degree from Tokyo Institute of Technology (Japan) in 1991. He was selected as an Academician of CAS in 2015. He is an adjunct professor of Tsinghua University (China) and a guest professor of Kyoto University (Japan). His research interests include molecular materials and devices. He has more than 700 refereed publications with over 40000 citations.
- DOI：10.1007/s10118-023-2952-0
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Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors[J]. 高分子科学（英文版）, 2023,41(5):652-670.

Yi-Fan Li, Yun-Long Guo, Yun-Qi Liu. Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors[J]. Chinese Journal of Polymer Science, 2023,41(5):652-670.
Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors[J]. 高分子科学（英文版）, 2023,41(5):652-670. DOI： 10.1007/s10118-023-2952-0.

Yi-Fan Li, Yun-Long Guo, Yun-Qi Liu. Recent Progress in Donor-Acceptor Type Conjugated Polymers for Organic Field-effect Transistors[J]. Chinese Journal of Polymer Science, 2023,41(5):652-670. DOI： 10.1007/s10118-023-2952-0.

摘要

We describe the recent progress in D-A conjugated polymers for OFETs from three aspects: (1) the modification of π-conjugated backbone, (2) the evolution of the polymerization methods and (3) the regulation of aggregate-state structure.

Abstract

The recent progress in the design and synthesis of high-performance donor-acceptor conjugated polymeric semiconducting materials is reviewed from the perspective of multiscale structures. The multiscale of conjugated polymers is from the primary one-dimensional polymer molecular scale to the secondary polymer-chains interaction scale, and then to the tertiary polymer aggregate scale. This review focuses on the design and synthesis of polymer molecules, proposes new classification rules, and rationally summarizes the design strategies and modulation methods of polymers. We describe the recent progress from these three aspects: (1) the modification of,π,-conjugated backbone, (2) the evolution of the polymerization methods, and (3) the regulation of aggregate-state structure.

关键词

Keywords

Conjugated polymersDonor-acceptorOrganic field-effect transistorsMultiscale optimization

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