Inkjet-Printed Organic Solar Cells and Perovskite Solar Cells: Progress, Challenges, and Prospect

Xing-Ze Chen; Qun Luo; Chang-Qi Ma

doi:10.1007/s10118-023-2961-z

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Inkjet-Printed Organic Solar Cells and Perovskite Solar Cells: Progress, Challenges, and Prospect

REVIEW | Updated：2023-07-18

- Inkjet-Printed Organic Solar Cells and Perovskite Solar Cells: Progress, Challenges, and Prospect
- Chinese Journal of Polymer Science Vol. 41, Issue 8, Pages: 1169-1197(2023)
- Affiliations：
  
  a.School of Nano-Tech and Nano-Bionics, University of Science and Technology of China, Hefei 230027, China
  b.i-Lab & Printable Electronics Research Center, Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou 215123, China
- Author bio：
  
  qluo2011@sinano.ac.cn (Q.L.)
  cqma2011@sinano.ac.cn (C.Q.M.)
- Funds：
- DOI：10.1007/s10118-023-2961-z
  CLC：
- Received：12 December 2022，
  
  Revised：2023-1-20，
  
  Accepted：31 January 2023，
  
  Online First：23 March 2023，
  
  Published：01 August 2023
- Accepted：
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Chen, X. Z.; Luo, Q.; Ma, C. Q. Inkjet-printed organic solar cells and perovskite solar cells: progress, challenges, and prospect. Chinese J. Polym. Sci. 2023, 41, 1169–1197

Xing-Ze Chen, Qun Luo, Chang-Qi Ma. Inkjet-Printed Organic Solar Cells and Perovskite Solar Cells: Progress, Challenges, and Prospect[J]. Chinese Journal of Polymer Science, 2023, 41(8): 1169-1197.
Chen, X. Z.; Luo, Q.; Ma, C. Q. Inkjet-printed organic solar cells and perovskite solar cells: progress, challenges, and prospect. Chinese J. Polym. Sci. 2023, 41, 1169–1197 DOI： 10.1007/s10118-023-2961-z.

Xing-Ze Chen, Qun Luo, Chang-Qi Ma. Inkjet-Printed Organic Solar Cells and Perovskite Solar Cells: Progress, Challenges, and Prospect[J]. Chinese Journal of Polymer Science, 2023, 41(8): 1169-1197. DOI： 10.1007/s10118-023-2961-z.

摘要

Abstract

In recent years

the power conversion efficiency of organic solar cells (OSCs) and perovskite (PVSCs) has increased to over 19% and 25%

respectively. Meanwhile

the long-term stability of OSCs and PVSCs was also significantly improved with a better understanding of the degradation mechanism and the improvement of materials

morphology

and interface stability. As both the efficiency and lifetime of solar cells are approaching the commercialization limit

fabrication methods for large-area OSCs and PVSCs that can be directly transferred from lab to fab become essential to promote the industrialization of OSCs and PVSCs. Compared with the coating methods

inkjet printing is a mature industrial technology with the advantages of random digital patterning

excellent precision and fast printing speed

which is considered to have great potential in solar cell fabrication. Many efforts have been devoted to developing inkjet-printed OSCs and PVSCs

and much progress has been achieved in the last few years. In this review

we first introduced the working principle of inkjet printing

the rheology requirements of inks

and the behaviors of the droplets. We then summarized the recent research progresses of the inkjet-printed OSCs and PVSCs to facilitate knowledge transfer between the two technologies. In the end

we gave a perspective on inkjet-printed OSCs and PVSCs.

关键词

Keywords

references

Ameri,T.;Khoram,P.;Min,J.;Brabec,C.J.Organicternarysolarcells:Areview. Adv. Mater. 2013 , 25 ,4245−4266..

Hou,J.;Inganas,O.;Friend,R.H.;Gao,F.Organicsolarcellsbasedonnon-fullereneacceptors. Nat. Mater. 2018 , 17 ,119−128..

Zhang,J.;Tan,H.S.;Guo,X.;Facchetti,A.;Yan,H.Materialinsightsandchallengesfornon-fullereneorganicsolarcellsbasedonsmallmolecularacceptors. Nat. Energy 2018 , 3 ,720−731..

Fukuda,K.;Yu,K.;Someya,T.Thefutureofflexibleorganicsolarcells. Adv. Energy Mater. 2020 , 10 ,2000765..

Kearns,D.;Calvin,M.Photovoltaiceffectandphotoconductivityinlaminatedorganicsystems. J. Phys. Chem. Lett. 1958 , 29 ,950−951..

Tang,C.W.Two-layerorganicphotovoltaiccell. Appl. Phys. Lett. 1986 , 48 ,183−185..

Yu,G.;Gao,J.;Hummelen,J.C.;Wudl,F.;Heeger,A.J.Polymerphotovoltaiccells:enhancedefficiencies via anetworkofinternaldonor-acceptorheterojunctions. Science 1995 , 270 ,1789−1791..

Cui,Y.;Xu,Y.;Yao,H.;Bi,P.;Hong,L.;Zhang,J.;Zu,Y.;Zhang,T.;Qin,J.;Ren,J.;Chen,Z.;He,C.;Hao,X.;Wei,Z.;Hou,J.Single-junctionorganicphotovoltaiccellwith19%efficiency. Adv. Mater. 2021 , 33 ,2102420..

Bi,P.;Zhang,S.;Ren,J.;Chen,Z.;Zheng,Z.;Cui,Y.;Wang,J.;Wang,S.;Zhang,T.;Li,J.;Xu,Y.;Qin,J.;An,C.;Ma,W.;Hao,X.;Hou,J.Ahigh-performancenonfusedwide-bandgapacceptorforversatilephotovoltaicapplications. Adv. Mater. 2022 , 34 ,2108090..

Kojima,A.;Teshima,K.;Shirai,Y.;Miyasaka,T.Organometalhalideperovskitesasvisible-lightsensitizersforphotovoltaiccells. J. Am. Chem. Soc. 2009 , 131 ,6050−6051..

Kim,H.S.;Lee,C.R.;Im,J.H.;Lee,K.B.;Moehl,T.;Marchioro,A.;Moon,S.J.;Humphry-Baker,R.;Yum,J.H.;Moser,J.E.;Gratzel,M.;Park,N.G.Leadiodideperovskitesensitizedall-solid-statesubmicronthinfilmmesoscopicsolarcellwithefficiencyexceeding9%. Sci. Rep. 2012 , 2 ,591..

Jiang,Q.;Zhao,Y.;Zhang,X.;Yang,X.;Chen,Y.;Chu,Z.;Ye,Q.;Li,X.;Yin,Z.;You,J.Surfacepassivationofperovskitefilmforefficientsolarcells. Nat. Photon. 2019 , 13 ,460−466..

Peng,J.;Kremer,F.;Walter,D.;Wu,Y.;Ji,Y.;Xiang,J.;Liu,W.;Duong,T.;Shen,H.;Lu,T.;Brink,F.;Zhong,D.;Li,L.;LeeCheongLem,O.;Liu,Y.;Weber,K.J.;White,T.P.;Catchpole,K.R.Centimetre-scaleperovskitesolarcellswithfillfactorsofmorethan86percent. Nature 2022 , 601 ,573−578..

Yoo,J.J.;Seo,G.;Chua,M.R.;Park,T.G.;Lu,Y.;Rotermund,F.;Kim,Y.K.;Moon,C.S.;Jeon,N.J.;Correa-Baena,J.P.;Bulović,V.;Shin,S.S.;Bawendi,M.G.;Seo,J.Efficientperovskitesolarcells via improvedcarriermanagement. Nature 2021 , 590 ,587−593..

Chen,X.;Huang,R.;Han,Y.;Zha,W.;Fang,J.;Lin,J.;Luo,Q.;Chen,Z.;Ma,C.Q.Balancingthemolecularaggregationandverticalphaseseparationinthepolymer:Nonfullereneblendfilmsenables13.09%efficiencyoforganicsolarcellswithinkjet-printedactivelayer. Adv. Energy Mater. 2022 , 12 ,2200044..

Eggers,H.;Schackmar,F.;Abzieher,T.;Sun,Q.;Lemmer,U.;Vaynzof,Y.;Richards,B.S.;Hernandez-Sosa,G.;Paetzold,U.W.Inkjet-printedmicrometer-thickperovskitesolarcellswithlargecolumnargrains. Adv. Energy Mater. 2020 , 10 ,1903184..

Yang,X.;Lin,Y.;Wu,T.;Yan,Z.;Chen,Z.;Kuo,H.C.;Zhang,R.Anoverviewontheprincipleofinkjetprintingtechniqueanditsapplicationinmicro-displayforaugmented/virtualrealities. Opto-Electr. Adv. 2022 , 5 ,210123−210123..

Sawa,M.;Fantuzzi,A.;Bombelli,P.;Howe,C.J.;Hellgardt,K.;Nixon,P.J.Electricitygenerationfromdigitallyprintedcyanobacteria. Nat. Commun. 2017 , 8 ,1327..

Han,G.D.;Bae,K.;Kang,E.H.;Choi,H.J.;Shim,J.H.Inkjetprintingformanufacturingsolidoxidefuelcells. ACS Energy Lett. 2020 , 5 ,1586−1592..

Sandler,N.;Maattanen,A.;Ihalainen,P.;Kronberg,L.;Meierjohann,A.;Viitala,T.;Peltonen,J.Inkjetprintingofdrugsubstancesanduseofporoussubstrates-towardsindividualizeddosing. J. Pharm. Sci. 2011 , 100 ,3386−3395..

Karunakaran,S.K.;Arumugam,G.M.;Yang,W.;Ge,S.;Khan,S.N.;Lin,X.;Yang,G.Recentprogressininkjet-printedsolarcells. J. Mater. Chem. A 2019 , 7 ,13873−13902..

Ganesan,S.;Mehta,S.;Gupta,D.Fullyprintedorganicsolarcells-areviewoftechniques,challengesandtheirsolutions. Opto-Electron. Rev. 2019 , 27 ,298−320..

Daly,R.;Harrington,T.S.;Martin,G.D.;Hutchings,I.M.Inkjetprintingforpharmaceutics—areviewofresearchandmanufacturing. Int. J. Pharm. 2015 , 494 ,554−567..

Wijshoff,H.Thedynamicsofthepiezoinkjetprintheadoperation. Phys. Rep. 2010 , 491 ,77−177..

Fromm,J.E.Numericalcalculationofthefluiddynamicsofdrop-on-demandjets. IBM J. Res. Dev. 1984 , 28 ,322−333..

Sumaiya,S.;Kardel,K.;ElShahat,A.Organicsolarcellbyinkjetprinting—anoverview. Technologies 2017 , 5 ,53..

Reis,N.;Ainsley,C.;Derby,B.Ink-jetdeliveryofparticlesuspensionsbypiezoelectricdropletejectors. J. Appl. Phys. 2005 , 97 ,094903..

Stow,C.D.;Hadfield,M.G.Anexperimentalinvestigationoffluid-flowresultingfromtheimpactofawaterdropwithanunyieldingdrysurface. Proc. R. Soc. Lond. A 1981 , 373 ,419−441..

Li,J.;Rossignol,F.;Macdonald,J.Inkjetprintingforbiosensorfabrication:Combiningchemistryandtechnologyforadvancedmanufacturing. Lab Chip 2015 , 15 ,2538−2558..

Corzo,D.;Almasabi,K.;Bihar,E.;Macphee,S.;Rosas-Villalva,D.;Gasparini,N.;Inal,S.;Baran,D.Digitalinkjetprintingofhigh-efficiencylarge-areanonfullereneorganicsolarcells. Adv. Mater. Technol. 2019 , 4 ,1900040..

Soltman,D.;Subramanian,V.Inkjet-printedlinemorphologiesandtemperaturecontrolofthecoffeeringeffect. Langmuir 2008 , 24 ,2224−2231..

Cherian,D.;Mitra,K.Y.;Hartwig,M.;Malinowski,P.E.;Baumann,R.R.Fabricationoforganicphotodetectorsusinginkjettechnologyanditscomparisontoconventionaldepositionprocesses. IEEE Sens. J. 2018 , 18 ,94−105..

Du,Z.H.;Zhou,H.;Yu,X.H.;Han,Y.C.Controllingthepolarityandviscosityofsmallmoleculeinktosuppressthecontactlinerecedingandcoffeeringeffectduringinkjetprinting. Colloids Surf., A 2020 , 602 ,125111..

Al-Milaji,K.N.;Secondo,R.R.;Ng,T.N.;Kinsey,N.;Zhao,H.Interfacialself-assemblyofcolloidalnanoparticlesindual-dropletinkjetprinting. Adv. Mater. Interfaces 2018 , 5 ,1701561..

Kuang,M.;Wang,L.;Song,Y.Controllableprintingdropletsforhigh-resolutionpatterns. Adv. Mater. 2014 , 26 ,6950−6958..

Matavž,A.;Frunză,R.C.;Drnovšek,A.;Bobnar,V.;Malič,B.Inkjetprintingofuniformdielectricoxidestructuresfromsol-gelinksbyadjustingthesolventcomposition. J. Mater. Chem. C 2016 , 4 ,5634−5641..

Jung,S.;Sou,A.;Banger,K.;Ko,D.H.;Chow,P.C.Y.;McNeill,C.R.;Sirringhaus,H.All-inkjet-printed,all-air-processedsolarcells. Adv. Energy Mater. 2014 , 4 ,1400432..

Lim,J.A.;Lee,W.H.;Lee,H.S.;Lee,J.H.;Park,Y.D.;Cho,K.Self-organizationofink-jet-printedtriisopropylsilylethynylpentacene via evaporation-inducedflowsinadryingdroplet. Adv. Funct. Mater. 2008 , 18 ,229−234..

Teichler,A.;Perelaer,J.;Schubert,U.S.Inkjetprintingoforganicelectronics—comparisonofdepositiontechniquesandstate-of-the-artdevelopments. J. Mater. Chem. C 2013 , 1 ,1910−1925..

Sempels,W.;DeDier,R.;Mizuno,H.;Hofkens,J.;Vermant,J.Auto-productionofbiosurfactantsreversesthecoffeeringeffectinabacterialsystem. Nat. Commun. 2013 , 4 ,1757..

Marin,V.;Holder,E.;Wienk,M.M.;Tekin,E.;Kozodaev,D.;Schubert,U.S.Ink-jetprintingofelectrondonor/acceptorblends:towardsbulkheterojunctionsolarcells. Macromol. Rapid Commun. 2005 , 26 ,319−324..

Hoth,C.N.;Choulis,S.A.;Schilinsky,P.;Brabec,C.J.Highphotovoltaicperformanceofinkjetprintedpolymer:fullereneblends. Adv. Mater. 2007 , 19 ,3973−3978..

Eggenhuisen,T.M.;Galagan,Y.;Biezemans,A.F.K.V.;Slaats,T.M.W.L.;Voorthuijzen,W.P.;Kommeren,S.;Shanmugam,S.;Teunissen,J.P.;Hadipour,A.;Verhees,W.J.H.;Veenstra,S.C.;Coenen,M.J.J.;Gilot,J.;Andriessen,R.;Groen,W.A.Highefficiency,fullyinkjetprintedorganicsolarcellswithfreedomofdesign. J. Mater. Chem. A 2015 , 3 ,7255−7262..

Corzo,D.;Bihar,E.;Alexandre,E.B.;Rosas-Villalva,D.;Baran,D.Inkengineeringoftransportlayersfor9.5%efficientall-printedsemitransparentnonfullerenesolarcells. Adv. Funct. Mater. 2020 , 31 ,2005763..

Jeong,J.A.;Lee,J.;Kim,H.;Kim,H.K.;Na,S.I.Ink-jetprintedtransparentelectrodeusingnano-sizeindiumtinoxideparticlesfororganicphotovoltaics. Sol. Energy Mater. Sol. Cells 2010 , 94 ,1840−1844..

Choi,K.H.;Jeong,J.A.;Kim,H.K.Dependenceofelectrical,optical,andstructuralpropertiesonthethicknessofIZTOthinfilmsgrownbylinearfacingtargetsputteringfororganicsolarcells. Sol. Energy Mater. Sol. Cells 2010 , 94 ,1822−1830..

Chang,Y.M.;Wang,L.;Su,W.F.Polymersolarcellswithpoly(3,4-ethylenedioxythiophene)astransparentanode. Org. Electron. 2008 , 9 ,968−973..

Na,S.I.;Park,D.W.;Kim,S.S.;Yang,S.Y.;Lee,K.;Lee,M.H.ITO-freeflexiblepolymersolarcellswithink-jet-printedAggrids. Semicond. Sci. Technol. 2012 , 27 ,125002..

Maisch,P.;Tam,K.C.;Lucera,L.;Egelhaaf,H.J.;Scheiber,H.;Maier,E.;Brabec,C.J.Inkjetprintedsilvernanowirepercolationnetworksaselectrodesforhighlyefficientsemitransparentorganicsolarcells. Org. Electron. 2016 , 38 ,139−143..

Kim,J.;Na,S.I.;Kim,H.K.InkjetprintingoftransparentInZnSnOconductingelectrodesfromnano-particleinkforprintableorganicphotovoltaics. Sol. Energy Mater. Sol. Cells 2012 , 98 ,424−432..

Galagan,Y.;Coenen,E.W.C.;Sabik,S.;Gorter,H.H.;Barink,M.;Veenstra,S.C.;Kroon,J.M.;Andriessen,R.;Blom,P.W.M.Evaluationofink-jetprintedcurrentcollectinggridsandbusbarsforITO-freeorganicsolarcells. Sol. Energy Mater. Sol. Cells 2012 , 104 ,32−38..

Lee,I.;Kim,G.W.;Yang,M.;Kim,T.S.SimultaneouslyenhancingthecohesionandelectricalconductivityofPEDOT:PSSconductivepolymerfilmsusingDMSOadditives. ACS Appl. Mater. Interfaces 2016 , 8 ,302−310..

Kim,J.Y.;Jung,J.H.;Lee,D.E.;Joo,J.Enhancementofelectricalconductivityofpoly(3,4-ethylenedioxythiophene)/poly(4-styrenesulfonate)byachangeofsolvents. Synth. Met. 2002 , 126 ,311..

Yamaguchi,H.;Aizawa,K.;Chonan,Y.;Komiyama,T.;Aoyama,T.;Sakai,E.;Qiu,J.;Sato,N.Highlyflexibleandconductiveglycerol-dopedPEDOT:PSSfilmspreparedunderanelectricfield. J. Electron. Mater. 2018 , 47 ,3370−3375..

Khasim,S.;Pasha,A.;Roy,A.S.;Parveen,A.;Badi,N.EffectofsecondarydopingusingsorbitolonstructureandtransportpropertiesofPEDOT-PSSthinfilms. J. Electron. Mater. 2017 , 46 ,4439−4447..

Kishi,N.;Kondo,Y.;Kunieda,H.;Hibi,S.;Sawada,Y.EnhancementofthermoelectricpropertiesofPEDOT:PSSthinfilmsbyadditionofanionicsurfactants. J. Mater. Sci. Mater. Electron. 2018 , 29 ,4030−4034..

Yeon,C.;Kim,G.;J;Yun,S.J.HighlyconductivePEDOT:PSStreatedbysodiumdodecylsulfateforstretchablefabricheaters. RSC Adv. 2017 , 7 ,5888−5897..

Lee,J.H.;Jeong,Y.R.;Lee,G.;Jin,S.W.;Lee,Y.H.;Hong,S.Y.;Park,H.;Kim,J.W.;Lee,S.S.;Ha,J.S.Highlyconductive,stretchable,andtransparentPEDOT:PSSelectrodesfabricatedwithtriblockcopolymeradditivesandacidtreatment. ACS Appl. Mater. Interfaces 2018 , 10 ,28027−28035..

Xia,Y.;Sun,K.;Ouyang,J.Solution-processedmetallicconductingpolymerfilmsastransparentelectrodeofoptoelectronicdevices. Adv. Mater. 2012 , 24 ,2436−2440..

Hau,S.K.;Yip,H.L.;Zou,J.;Jen,A.K.Y.Indiumtinoxide-freesemi-transparentinvertedpolymersolarcellsusingconductingpolymerasbothbottomandtopelectrodes. Org. Electron. 2009 , 10 ,1401−1407..

Zhou,Y.;Cheun,H.;Choi,S.;Potscavage,W.J.;Fuentes-Hernandez,C.;Kippelen,B.Indiumtinoxide-freeandmetal-freesemitransparentorganicsolarcells. Appl. Phys. Lett. 2010 , 97 ,153304..

Galagan,Y.;Zimmermann,B.;Coenen,E.W.C.;Jørgensen,M.;Tanenbaum,D.M.;Krebs,F.C.;Gorter,H.;Sabik,S.;Slooff,L.H.;Veenstra,S.C.;Kroon,J.M.;Andriessen,R.CurrentcollectinggridsforITO-freesolarcells. Adv. Energy Mater. 2012 , 2 ,103−110..

Neophytou,M.;Hermerschmidt,F.;Savva,A.;Georgiou,E.;Choulis,S.A.Highlyefficientindiumtinoxide-freeorganicphotovoltaicsusinginkjet-printedsilvernanoparticlecurrentcollectinggrids. Appl. Phys. Lett. 2012 , 101 ,193302..

Neophytou,M.;Georgiou,E.;Fyrillas,M.M.;Choulis,S.A.TwostepsinteringprocessandmetalgriddesignoptimizationforhighlyefficientITOfreeorganicphotovoltaics. Sol. Energy Mater. Sol. Cells 2014 , 122 ,1−7..

Kim,Y.H.;Sachse,C.;Machala,M.L.;May,C.;Müller-Meskamp,L.;Leo,K.HighlyconductivePEDOT:PSSelectrodewithoptimizedsolventandthermalpost-treatmentforITO-freeorganicsolarcells. Adv. Funct. Mater. 2011 , 21 ,1076−1081..

Huang,Y.C.;Hsu,F.H.;Cha,H.C.;Chuang,C.M.;Tsao,C.S.;Chen,C.Y.High-performanceITO-freespray-processedpolymersolarcellswithincorporatingink-jetprintedgrid. Org. Electron. 2013 , 14 ,2809−2817..

Zhang,Z.L.;Si,T.T.;Liu,J.Controllableassemblyofahierarchicalmultiscalearchitecturebasedonsilvernanoparticlegrids/nanowiresforflexibleorganicsolarcells. Nanotechnology 2018 , 29 ,11..

Georgiou,E.;Choulis,S.A.;Hermerschmidt,F.;Pozov,S.M.;Burgues-Ceballos,I.;Christodoulou,C.;Schider,G.;Kreissl,S.;Ward,R.;List-Kratochvil,E.J.W.;Boeffel,C.Printedcoppernanoparticlemetalgridsforcost-effectiveITO-freesolutionprocessedsolarcells. Sol. RRL 2018 , 2 ,1700192..

Pan,W.;Han,Y.;Wang,Z.;Gong,C.;Guo,J.;Lin,J.;Luo,Q.;Yang,S.;Ma,C.Q.Anefficiencyof14.29%and13.08%for1cm 2 and4cm 2 flexibleorganicsolarcellsenabledbysol-gelZnOandZnOnanoparticlebilayerelectrontransportinglayers. J. Mater. Chem. A 2021 , 9 ,16889−16897..

Guo,J.B.;Han,Y.F.;Xu,Z.H.;Zha,W.S.;Fang,J.;Luo,Q.;Liu,L.Q.;Ma,C.Q.MonodispersedZnOnanoinkandultra-smoothlarge-areaZnOfilmsforhighperformanceandstableorganicsolarcells. Flex. Print. Electron. 2022 , 7 ,025013..

Singh,A.;Gupta,S.K.;Garg,A.Invertedpolymerbulkheterojunctionsolarcellswithink-jetprintedelectrontransportandactivelayers. Org. Electron. 2016 , 35 ,118−127..

Sacramento,A.;Ramirez-Como,M.;Balderrama,V.S.;Garduno,S.I.;Estrada,M.;Marsal,L.F.InvertedpolymersolarcellsusinginkjetprintedZnOaselectrontransportlayer:characterizationanddegradationstudy. IEEE J. Electron Devices Soc. 2020 , 8 ,413−420..

Kommeren,S.;Coenen,M.J.J.;Eggenhuisen,T.M.;Slaats,T.W.L.;Gorter,H.;Groen,P.CombiningsolventsandsurfactantsforinkjetprintingPEDOT:PSSonP3HT/PCBMinorganicsolarcells. Org. Electron. 2018 , 61 ,282−288..

Singh,A.;Gupta,S.K.;Garg,A.InkjetprintingofNiOfilmsandintegrationasholetransportinglayersinpolymersolarcells. Sci. Rep. 2017 , 7 ,1775..

Jiang,Y.;Dong,X.;Sun,L.;Liu,T.;Qin,F.;Xie,C.;Jiang,P.;Hu,L.;Lu,X.;Zhou,X.;Meng,W.;Li,N.;Brabec,C.J.;Zhou,Y.Analcohol-dispersedconductingpolymercomplexforfullyprintableorganicsolarcellswithimprovedstability. Nat. Energy 2022 , 7 ,352−359..

Lamont,C.A.;Eggenhuisen,T.M.;Coenen,M.J.J.;Slaats,T.W.L.;Andriessen,R.;Groen,P.Tuningtheviscosityofhalogenfreebulkheterojunctioninksforinkjetprintedorganicsolarcells. Org. Electron. 2015 , 17 ,107−114..

Aernouts,T.;Aleksandrov,T.;Girotto,C.;Genoe,J.;Poortmans,J.Polymerbasedorganicsolarcellsusingink-jetprintedactivelayers. Appl. Phys. Lett. 2008 , 92 ,033306..

Hoth,C.N.;Schilinsky,P.;Choulis,S.A.;Brabec,C.J.Printinghighlyefficientorganicsolarcells. Nano Lett. 2008 , 8 ,2806−2813..

Teichler,A.;Eckardt,R.;Hoeppener,S.;Friebe,C.;Perelaer,J.;Senes,A.;Morana,M.;Brabec,C.J.;Schubert,U.S.Combinatorialscreeningofpolymer:fullereneblendsfororganicsolarcellsbyinkjetprinting. Adv. Energy Mater. 2011 , 1 ,105−114..

Eom,S.H.;Park,H.;Mujawar,S.H.;Yoon,S.C.;Kim,S.S.;Na,S.I.;Kang,S.J.;Khim,D.;Kim,D.Y.;Lee,S.H.Highefficiencypolymersolarcells via sequentialinkjet-printingofPEDOT:PSSandP3HT:PCBMinkswithadditives. Org. Electron. 2010 , 11 ,1516−1522..

Hoth,C.N.;Choulis,S.A.;Schilinsky,P.;Brabec,C.J.Ontheeffectofpoly(3-hexylthiophene)regioregularityoninkjetprintedorganicsolarcells. J. Mater. Chem. 2009 , 19 ,5398..

Ganesan,S.;Gollu,S.R.;Alamkhan,J.;Kushwaha,A.;Gupta,D.InkjetprintingofzincoxideandP3HT:ICBAinambientconditionsforinvertedbulkheterojunctionsolarcells. Opt. Mater. 2019 , 94 ,430−435..

Eggenhuisen,T.M.;Galagan,Y.;Coenen,E.W.C.;Voorthuijzen,W.P.;Slaats,M.W.L.;Kommeren,S.A.;Shanmuganam,S.;Coenen,M.J.J.;Andriessen,R.;Groen,W.A.Digitalfabricationoforganicsolarcellsbyinkjetprintingusingnon-halogenatedsolvents. Sol. Energy Mater. Sol. Cells 2015 , 134 ,364−372..

Perkhun,P.;Köntges,W.;Pourcin,F.;Esteoulle,D.;Barulina,E.;Yoshimoto,N.;Pierron,P.;Margeat,O.;Videlot-Ackermann,C.;Bharwal,A.K.;Duché,D.;Herrero,C.R.;Gonzales,C.;Guerrero,A.;Bisquert,J.;Schröder,R.R.;Pfannmöller,M.;BenDkhil,S.;Simon,J.J.;Ackermann,J.High-efficiencydigitalinkjet-printednon-fullerenepolymerblendsusingnon-halogenatedsolvents. Adv. Energy Sustain. Res. 2021 , 2 ,2000086..

Lan,S.;Zhong,J.;Wang,X.Impactofinkjetprintingparametersonthemorphologyanddeviceperformanceoforganicphotovoltaics. J. Phys. D: Appl. Phys. 2021 , 54 ,465105..

Wang,Y.;Luo,Q.;Wu,N.;Wang,Q.;Zhu,H.;Chen,L.;Li,Y.Q.;Luo,L.;Ma,C.Q.Solution-processedMoO 3 :PEDOT:PSShybridholetransportinglayerforinvertedpolymersolarcells. ACS Appl. Mater. Interfaces 2015 , 7 ,7170−7179..

Ji,G.;Wang,Y.;Luo,Q.;Han,K.;Xie,M.;Zhang,L.;Wu,N.;Lin,J.;Xiao,S.;Li,Y.Q.;Luo,L.Q.;Ma,C.Q.Fullycoatedsemitransparentorganicsolarcellswithadoctor-blade-coatedcompositeanodebufferlayerofphosphomolybdicacidandPEDOT:PSSandaspray-coatedsilvernanowiretopelectrode. ACS Appl. Mater. Interfaces 2018 , 10 ,943−954..

Li,D.;Lai,W.Y.;Zhang,Y.Z.;Huang,W.Printabletransparentconductivefilmsforflexibleelectronics. Adv. Mater. 2018 , 30 ,1704738..

Hermerschmidt,F.;Choulis,S.A.;List-Kratochvil,E.J.W.Implementinginkjet-printedtransparentconductiveelectrodesinsolution-processedorganicelectronics. Adv. Mater. Technol. 2019 , 4 ,1800474..

Galagan,Y.;Shanmugam,S.;Teunissen,J.P.;Eggenhuisen,T.M.;Biezemans,A.F.K.V.;VanGijseghem,T.;Groen,W.A.;Andriessen,R.Solutionprocessingofbackelectrodesfororganicsolarcellswithinvertedarchitecture. Sol. Energy Mater. Sol. Cells 2014 , 130 ,163−169..

Georgiou,E.;Savva,A.;Neophytou,M.;Hermerschmidt,F.;Demosthenous,T.;Choulis,S.A.Evaporation-freeinvertedorganicphotovoltaicsusingamixtureofsilvernanoparticleinkformulationsforsolution-processedtopelectrodes. Appl. Phys. Lett. 2014 , 105 ,233901..

Lu,H.;Lin,J.;Wu,N.;Nie,S.;Luo,Q.;Ma,C.Q.;Cui,Z.Inkjetprintedsilvernanowirenetworkastopelectrodeforsemi-transparentorganicphotovoltaicdevices. Appl. Phys. Lett. 2015 , 106 ,093302..

Finn,D.J.;Lotya,M.;Coleman,J.N.Inkjetprintingofsilvernanowirenetworks. ACS Appl. Mater. Interfaces 2015 , 7 ,9254−9261..

Park,E.K.;Kim,J.H.;Lee,D.H.;Kim,K.S.;Kal,J.H.;Hahn,J.S.;Kim,Y.S.Allink-jetprintedP3HT:PCBMorganicsolarcellsonITO-coatedglasssubstrate. J. Nanosci. Nanotechnol. 2015 , 15 ,8790−8796..

Maisch,P.;Tam,K.C.;Schilinsky,P.;Egelhaaf,H.J.;Brabec,C.J.Shyorganicphotovoltaics:digitallyprintedorganicsolarmoduleswithhiddeninterconnects. Sol. RRL 2018 , 2 ,1800005..

Mitra,K.Y.;Alalawe,A.;Voigt,S.;Boeffel,C.;Baumann,R.R.Manufacturingofallinkjet-printedorganicphotovoltaiccellarraysandevaluatingtheirsuitabilityforflexibleelectronics. Micromachines 2018 , 9 ,642..

Bihar,E.;Corzo,D.;Hidalgo,T.C.;Rosas-Villalva,D.;Salama,K.N.;Inal,S.;Baran,D.Fullyinkjet-printed,ultrathinandconformableorganicphotovoltaicsaspowersourcebasedoncross-linkedPEDOT:PSSelectrodes. Adv. Mater. Technol. 2020 , 5 ,2000226..

Patil,B.R.;Shanmugam,S.;Teunissen,J.P.;Galagan,Y.All-solutionprocessedorganicsolarcellswithtopillumination. Org. Electron. 2015 , 21 ,40−46..

Wei,Z.;Chen,H.;Yan,K.;Yang,S.InkjetprintingandinstantchemicaltransformationofaCH 3 NH 3 PbI 3 /nanocarbonelectrodeandinterfaceforplanarperovskitesolarcells. Angew. Chem. Int. Ed. 2014 , 53 ,13239−13243..

Li,S.G.;Jiang,K.J.;Su,M.J.;Cui,X.P.;Huang,J.H.;Zhang,Q.Q.;Zhou,X.Q.;Yang,L.M.;Song,Y.L.InkjetprintingofCH 3 NH 3 PbI 3 onamesoscopicTiO 2 filmforhighlyefficientperovskitesolarcells. J. Mater. Chem. A 2015 , 3 ,9092−9097..

Chalkias,D.A.;Mourtzikou,A.;Katsagounos,G.;Karavioti,A.;Kalarakis,A.N.;Stathatos,E.Suppressionofcoffee-ringeffectinair-processedinkjet-printedperovskitelayertowardthefabricationofefficientlarge-sizedall-printedphotovoltaics:aperovskiteprecursorinkconcentrationregulationstrategy. Sol. RRL 2022 , 6 ,2200196..

Gheno,A.;Huang,Y.;Bouclé,J.;Ratier,B.;Rolland,A.;Even,J.;Vedraine,S.Towardhighlyefficientinkjet-printedperovskitesolarcellsfullyprocessedunderambientconditionsandatlowtemperature. Sol. RRL 2018 , 2 ,1800191..

Zhang,L.H.;Chen,S.;Wang,X.Z.;Wang,D.;Li,Y.;Ai,Q.;Sun,X.Y.;Chen,J.B.;Li,Y.;Jiang,X.Z.;Yang,S.H.;Xu,B.M.Ambientinkjet-printedhigh-efficiencyperovskitesolarcells:manipulatingthespreadingandcrystallizationbehaviorsofpicoliterperovskitedroplets. Sol. RRL 2021 , 5 ,2100106..

Hashmi,S.G.;Martineau,D.;Li,X.;Ozkan,M.;Tiihonen,A.;Dar,M.I.;Sarikka,T.;Zakeeruddin,S.M.;Paltakari,J.;Lund,P.D.;Grätzel,M.Airprocessedinkjetinfiltratedcarbonbasedprintedperovskitesolarcellswithhighstabilityandreproducibility. Adv. Mater. Technol. 2017 , 2 ,1600183..

Pathak,C.S.;Paramasivam,G.;Mathies,F.;Hirselandt,K.;Schroder,V.;Maus,O.;Dagar,J.;Klimm,C.;Unger,E.;Visoly-Fisher,I.PTB7asanink-additiveforspin-coatedversusinkjet-printedperovskitesolarcells. ACS Appl. Energy Mater. 2022 , 5 ,4085−4095..

Li,Z.;Li,P.;Chen,G.;Cheng,Y.;Pi,X.;Yu,X.;Yang,D.;Han,L.;Zhang,Y.;Song,Y.Inkengineeringofinkjetprintingperovskite. ACS Appl. Mater. Interfaces 2020 , 12 ,39082−39091..

Wilk,B.;Öz,S.;Radicchi,E.;Ünlü,F.;Ahmad,T.;Herman,A.P.;Nunzi,F.;Mathur,S.;Kudrawiec,R.;Wojciechowski,K.Greensolvent-basedperovskiteprecursordevelopmentforink-jetprintedflexiblesolarcells. ACS Sustain. Chem. Eng 2021 , 9 ,3920−3930..

Liang,C.;Li,P.;Gu,H.;Zhang,Y.;Li,F.;Song,Y.;Shao,G.;Mathews,N.;Xing,G.One-stepinkjetprintedperovskiteinairforefficientlightharvesting. Sol. RRL 2018 , 2 ,1700217..

Mathies,F.;Abzieher,T.;Hochstuhl,A.;Glaser,K.;Colsmann,A.;Paetzold,U.W.;Hernandez-Sosa,G.;Lemmer,U.;Quintillaa,A.Multipassinkjetprintedplanarmethylammoniumleadiodideperovskitesolarcells. J. Mater. Chem. A 2016 , 4 ,19207−19213..

Huckaba,A.J.;Lee,Y.;Xia,R.;Paek,S.;Bassetto,V.C.;Oveisi,E.;Lesch,A.;Kinge,S.;Dyson,P.J.;Girault,H.;Nazeeruddin,M.K.Inkjet-printedmesoporousTiO 2 andperovskitelayersforhighefficiencyperovskitesolarcells. Energy Technol. 2019 , 7 ,317−324..

Schackmar,F.;Eggers,H.;Frericks,M.;Richards,B.S.;Lemmer,U.;Hernandez-Sosa,G.;Paetzold,U.W.Perovskitesolarcellswithall-inkjet-printedabsorberandchargetransportlayers. Adv. Mater. Technol. 2021 , 6 ,2000271..

Schlisske,S.;Mathies,F.;Busko,D.;Strobel,N.;Rodlmeier,T.;Richards,B.S.;Lemmer,U.;Paetzold,U.W.;Hernandez-Sosa,G.;Klampaftis,E.Designandcolorflexibilityforinkjet-printedperovskitephotovoltaics. ACS Appl. Energy Mater. 2019 , 2 ,764−769..

Hou,Y.;Xie,C.;Radmilovic,V.V.;Puscher,B.;Wu,M.;Heumuller,T.;Karl,A.;Li,N.;Tang,X.;Meng,W.;Chen,S.;Osvet,A.;Guldi,D.;Spiecker,E.;Radmilovic,V.R.;Brabec,C.J.Assemblingmesoscale-structuredorganicinterfacesinperovskitephotovoltaics. Adv. Mater. 2019 , 31 ,1806516..

Xie,C.;Heumuller,T.;Gruber,W.;Tang,X.;Classen,A.;Schuldes,I.;Bidwell,M.;Spath,A.;Fink,R.H.;Unruh,T.;McCulloch,I.;Li,N.;Brabec,C.J.Overcomingefficiencyandstabilitylimitsinwater-processingnanoparticularorganicphotovoltaicsbyminimizingmicrostructuredefects. Nat. Commun. 2018 , 9 ,5335..

Manger,F.;Marlow,P.;Fischer,K.;Nöller,M.;Sprau,C.;Colsmann,A.Organicsolarcells:electrostaticstabilizationoforganicsemiconductornanoparticledispersionsbyelectricaldoping. Adv. Funct. Mater. 2022 , 32 ,2202566..

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