Biomimetic Modification of Super-wetting Electrospun Poly(vinylidene fluoride) Porous Fibers with Organic Dyes and Heavy Metal Ions Adsorption, Oil/Water Separation, and Sterilization Performances Toward Wastewater Treatment

De-Xiang Sun; Xiao-Lei Liao; Nan Zhang; Ting Huang; Yan-Zhou Lei; Xiao-Ling Xu; Yong Wang

doi:10.1007/s10118-022-2714-4

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Biomimetic Modification of Super-wetting Electrospun Poly(vinylidene fluoride) Porous Fibers with Organic Dyes and Heavy Metal Ions Adsorption, Oil/Water Separation, and Sterilization Performances Toward Wastewater Treatment

RESEARCH ARTICLE | Updated：2022-06-22

- Biomimetic Modification of Super-wetting Electrospun Poly(vinylidene fluoride) Porous Fibers with Organic Dyes and Heavy Metal Ions Adsorption, Oil/Water Separation, and Sterilization Performances Toward Wastewater Treatment
- Chinese Journal of Polymer Science Vol. 40, Issue 7, Pages: 738-753(2022)
- Affiliations：
  
  a.School of Materials Science & Engineering, Key Laboratory of Advanced Technologies of Materials (Ministry of Education), Southwest Jiaotong University, Chengdu 610031, China
  b.Analytical and Testing Center, Southwest Jiaotong University, Chengdu 610031, China
- Author bio：
  
  sanyenan@163.com (N.Z.)
  yongwang1976@swjtu.edu.cn (Y.W.)
- Funds：
- DOI：10.1007/s10118-022-2714-4
  CLC：
- Received：01 January 2022，
  
  Revised：2022-1-23，
  
  Accepted：08 February 2022，
  
  Online First：20 May 2022，
  
  Published：01 July 2022
- Accepted：
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Sun, D. X.; Liao, X. L.; Zhang, N.; Huang, T.; Lei, Y. Z.; Xu, X. L.; Wang, Y. Biomimetic modification of super-wetting electrospun poly(vinylidene fluoride) porous fibers with organic dyes and heavy metal ions adsorption, oil/water separation, and sterilization performances toward wastewater treatment. Chinese J. Polym. Sci. 2022, 40, 738–753

De-Xiang Sun, Xiao-Lei Liao, Nan Zhang, et al. Biomimetic Modification of Super-wetting Electrospun Poly(vinylidene fluoride) Porous Fibers with Organic Dyes and Heavy Metal Ions Adsorption, Oil/Water Separation, and Sterilization Performances Toward Wastewater Treatment[J]. Chinese Journal of Polymer Science, 2022, 40(7): 738-753.
Sun, D. X.; Liao, X. L.; Zhang, N.; Huang, T.; Lei, Y. Z.; Xu, X. L.; Wang, Y. Biomimetic modification of super-wetting electrospun poly(vinylidene fluoride) porous fibers with organic dyes and heavy metal ions adsorption, oil/water separation, and sterilization performances toward wastewater treatment. Chinese J. Polym. Sci. 2022, 40, 738–753 DOI： 10.1007/s10118-022-2714-4.

De-Xiang Sun, Xiao-Lei Liao, Nan Zhang, et al. Biomimetic Modification of Super-wetting Electrospun Poly(vinylidene fluoride) Porous Fibers with Organic Dyes and Heavy Metal Ions Adsorption, Oil/Water Separation, and Sterilization Performances Toward Wastewater Treatment[J]. Chinese Journal of Polymer Science, 2022, 40(7): 738-753. DOI： 10.1007/s10118-022-2714-4.

摘要

The fibrous membranes exhibited switchable superhydrophilicity and superlipophilicity characteristics

excellent adsorption abilities toward organic dyes

heavy metal ions

and oils. Specifically

the membrane could rapidly remove the trace MB when water flowed through the membrane. The membrane also exhibited excellent sterilization performances and light-to-heat conversion ability.

Abstract

Polymeric membranes with the integration of various functional performances toward wastewater treatment are urgently required. However

most of the polymeric membranes only exhibit a single function of highly efficiently removing one kind of pollutants. In this work

a biomimetic modification method was introduced to tailor the chemical and topological structure of the porous poly(vinylidene fluoride) (PVDF) fibers prepared by electrospinning. The polydopamine (PDA) nanoparticles were homogeneously introduced onto the surface of PVDF porous fibers

via

precisely tailoring the concentration of dopamine

which endowed the fibers with more polar groups and bigger roughness but did not destroy the crystalline structures. The fibrous membranes exhibited switchable superhydrophilicity and superlipophilicity characteristics

excellent adsorption abilities toward organic dyes

heavy metal ions and oils. The highest adsorption capacities achieved 917.4 mg/g toward methylene blue (MB)

42.6 mg/g toward Cr(VI) and 74.6 g/g toward silicone oil

respectively. Specifically

the membrane could rapidly remove the trace MB when water flowed through the membrane. The membrane also exhibited excellent sterilization performances

and the bacterial eliminating rate achieved 99.9% for the

E. coli

and

S. aureus.

The excellent light-to-heat conversion ability endowed the membrane with the self-heating ability

furtherly intensifying the wastewater treatment efficiency. This work confirms that the PDA nanoparticles-decorated PVDF porous fibers might be the new generation adsorbents used in wastewater treatment.

关键词

Keywords

references

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