Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)

Liang-Qing Zhang; Shu-Gui Yang; Jing-Han Zhang; Ke-Peng Zhong; Zhong-Guo Zhao; Yan-Hui Chen; Jun Lei; Qiu-Yu Zhang; Zhong-Ming Li

doi:10.1007/s10118-022-2672-x

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Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)

RESEARCH ARTICLE | Updated：2022-03-23

- Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)
- Chinese Journal of Polymer Science Vol. 40, Issue 3, Pages: 290-298(2022)
- Affiliations：
  
  a.College of Material Science and Engineering, Xi’an University of Science and Technology, Xi’an 710054, China
  b.State Key Laboratory for Mechanical Behaviour of Materials, Shaanxi International Research Center for Soft Materials, Xi’an Jiaotong University, Xi’an 710049, China
  c.School of Chemistry and Chemical Engineering, Shaanxi Key Laboratory of Macromolecular Science and Technology, Key Laboratory of Special Functional and Smart Polymer Materials of Ministry of Industry and Information Technology, Northwestern Polytechnical University, Xi’an 710072, China
  d.National and Local Engineering Laboratory for Slag Comprehensive Utilization and Environment Technology, School of Materials Science and Engineering, Shaanxi University of Technology, Hanzhong 723000, China
  e.College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu 610065, China
- Author bio：
  
  yanhuichen@nwpu.edu.cn
- Funds：
- DOI：10.1007/s10118-022-2672-x
  CLC：
- Received：09 August 2021，
  
  Revised：2021-11-2，
  
  Accepted：23 November 2021，
  
  Online First：15 January 2022，
  
  Published：01 March 2022
- Accepted：
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Zhang, L. Q.; Yang, S. G.; Zhang, J. H.; Zhong, K. P.; Zhao, Z. G.; Chen, Y. H.; Lei, J.; Zhang, Q. Y.; Li, Z. M. Insight into the excellent tribological performance of highly oriented poly(phenylene sulfide). Chinese J. Polym. Sci. 2022, 40, 290–298

Liang-Qing Zhang, Shu-Gui Yang, Jing-Han Zhang, et al. Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)[J]. Chinese Journal of Polymer Science, 2022, 40(3): 290-298.
Zhang, L. Q.; Yang, S. G.; Zhang, J. H.; Zhong, K. P.; Zhao, Z. G.; Chen, Y. H.; Lei, J.; Zhang, Q. Y.; Li, Z. M. Insight into the excellent tribological performance of highly oriented poly(phenylene sulfide). Chinese J. Polym. Sci. 2022, 40, 290–298 DOI： 10.1007/s10118-022-2672-x.

Liang-Qing Zhang, Shu-Gui Yang, Jing-Han Zhang, et al. Insight into the Excellent Tribological Performance of Highly Oriented Poly(phenylene sulfide)[J]. Chinese Journal of Polymer Science, 2022, 40(3): 290-298. DOI： 10.1007/s10118-022-2672-x.

摘要

Abstract

Achieving low friction and wear of poly(phenylene sulfide) (PPS) without using fillers or blending is a challenging task

but one of considerable practical importance. Here we describe how neat PPS with high tribological performance is achieved by manipulating processing parameters (pressure

flow and temperature). The key to achieving high tribological performance is comparatively high molecular chain orientation

realized in neat PPS

at high shear rates and low pressure. The friction coefficient and wear rate are as low as ~0.3 and ~10

‒6

·N

‒1

·m

‒1

respectively

which break the record for neat PPS. These values are even better than those for PPS-based blends and comparable to PPS composites. Further studies show

for the first time

that wear rate decreases exponentially with increasing molecular chain orientation

prompting us to revise the classical Archard’s law by including the effect of molecular chain orientation. These ﬁndings open the possibility of using neat PPS in highly demanding tribological applications.

关键词

Keywords

references

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