Multifunctional Templating Strategy for Fabrication of Fe,N-Codoped Hierarchical Porous Carbon Nanosheets

Yu-heng Lu; You-chen Tang; Ru-liang Liu; Chuan-fa Li; Shao-hong Liu; You-long Zhu; Ding-cai Wu

doi:10.1007/s10118-022-2656-x

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Multifunctional Templating Strategy for Fabrication of Fe,N-Codoped Hierarchical Porous Carbon Nanosheets

Rapid Communication | Updated：2021-11-18

- Multifunctional Templating Strategy for Fabrication of Fe,N-Codoped Hierarchical Porous Carbon Nanosheets
- Chinese Journal of Polymer Science Vol. 40, Issue 1, Pages: 2-6(2022)
- Affiliations：
  
  Key Laboratory for Polymeric Composite & Functional Materials of Ministry of Education, School of Chemistry, Sun Yat-sen University, Guangzhou 510006, China
- Author bio：
  
  liuruliang0402@163.com (R.L.L.)
  liushh27@mail.sysu.edu.cn (S.H.L.)
  wudc@mail.sysu.edu.cn (D.C.W.)
- Funds：
  
  This work was financially supported by the National Natural Science Foundation of China (Nos. 51925308 and 51872336), the Leading Scientific, Technical and Innovation Talents of Guangdong Special Support Program (No. 2017TX04C248), the Pearl River Talent Plan of Guangdong (No. 2017GC010612), Natural Science Foundation of Guangdong (No. 2021A1515011617), the Fundamental Research Funds for the Central Universities (No. 20lgzd18), and the Science and Technology Program of Guangzhou (Nos. 202102021111 and 202002020041).
- DOI：10.1007/s10118-022-2656-x
  CLC：
- Received：08 September 2021，
  
  Revised：2021-10-17，
  
  Accepted：20 October 2021，
  
  Online First：18 November 2021，
  
  Published：01 January 2022
- Accepted：
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Lu, Y. H.; Tang, Y. C.; Liu, R. L.; Li, C. F.; Liu, S. H.; Zhu, Y. L.; Wu, D. C. Multifunctional templating strategy for fabrication of Fe,N-codoped hierarchical porous carbon nanosheets. Chinese J. Polym. Sci. 2022, 40, 2–6

Yu-heng Lu, You-chen Tang, Ru-liang Liu, et al. Multifunctional Templating Strategy for Fabrication of Fe,N-Codoped Hierarchical Porous Carbon Nanosheets[J]. Chinese Journal of Polymer Science, 2022, 40(1): 2-6.
Lu, Y. H.; Tang, Y. C.; Liu, R. L.; Li, C. F.; Liu, S. H.; Zhu, Y. L.; Wu, D. C. Multifunctional templating strategy for fabrication of Fe,N-codoped hierarchical porous carbon nanosheets. Chinese J. Polym. Sci. 2022, 40, 2–6 DOI： 10.1007/s10118-022-2656-x.

Yu-heng Lu, You-chen Tang, Ru-liang Liu, et al. Multifunctional Templating Strategy for Fabrication of Fe,N-Codoped Hierarchical Porous Carbon Nanosheets[J]. Chinese Journal of Polymer Science, 2022, 40(1): 2-6. DOI： 10.1007/s10118-022-2656-x.

摘要

Abstract

Due to the unique physical and chemical merits including excellent electrical conductivity

superior chemical stability

and tunable carbon framework

two-dimensional (2D) porous carbon nanosheets have drawn increasing research interest and demonstrated promising potentials in various applications. However

regulating the nanostructure of 2D porous carbon nanosheets by facile and efficient strategies remains a great challenge. Herein

we develop a new strategy to construct Fe

N-codoped hierarchical porous carbon nanosheets (Fe-N-HPCNS) by using 2D Fe-Zn layered double hydroxides (Fe-Zn-LDH) as multifunctional templates. Fe-Zn-LDH could functionalize not only as 2D structure directing agents but also as ternary hierarchical porogens for micro-

meso- and macropores and

in situ

Fe dopants. This multifunctional templating strategy toward 2D porous carbon nanosheets can improve the utilization of templates and shows great advantages against conventional procedures that additional porogens and/or dopants are often needed.

关键词

Keywords

references

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