A Mechanically Strong Conductive Hydrogel Reinforced by Diaminotriazine Hydrogen Bonding

Qian Wu; Bing Xu; Jun-jie Wei; Qing Wang; Qi-gang Wang; Wen-guang Liu

doi:10.1007/s10118-017-1960-3

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A Mechanically Strong Conductive Hydrogel Reinforced by Diaminotriazine Hydrogen Bonding

Papers | Updated：2021-02-18

- A Mechanically Strong Conductive Hydrogel Reinforced by Diaminotriazine Hydrogen Bonding
- Chinese Journal of Polymer Science Vol. 35, Issue 10, Pages: 1222-1230(2017)
- Affiliations：
  
  a.School of Materials Science and Engineering, Tianjin Key Laboratory of Composite and Functional Materials, Tianjin University, Tianjin 300350, China
  b.School of Chemical Science and Engineering, Tongji University, Shanghai 200092, China
- Author bio：
  
  Wen-guang Liu (刘文广), E-mail:wgliu@tju.edu.cn
- Funds：
- DOI：10.1007/s10118-017-1960-3
  CLC：
- Received：21 March 2017，
  
  Revised：2017-4-7，
  
  Accepted：11 April 2017，
  
  Published：05 October 2017
- Accepted：
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Qian Wu, Bing Xu, Jun-jie Wei, et al. A Mechanically Strong Conductive Hydrogel Reinforced by Diaminotriazine Hydrogen Bonding[J]. Chinese Journal of Polymer Science, 2017, 35(10): 1222-1230.
DOI：

Qian Wu, Bing Xu, Jun-jie Wei, et al. A Mechanically Strong Conductive Hydrogel Reinforced by Diaminotriazine Hydrogen Bonding[J]. Chinese Journal of Polymer Science, 2017, 35(10): 1222-1230. DOI： 10.1007/s10118-017-1960-3.

摘要

Abstract

Over the past decades

the urgent need for high strength conductive hydrogels in diverse applications has motivated an unremitting effort to combine the improved mechanical properties of hydrogels with conductive performances. In this work

high strength conductive hydrogels intensified with intermolecular hydrogen bonding are fabricated by

in situ

mixing poly(2-vinyl-4

6-diamino-1

5-triazine-

-polyethylene glycol diacrylates) (PVDT-PEGDA) hydrogels with poly(3

4-ethylenedioxythiophene)-poly(styrenesulfonate) (PEDOT/PSS). The conductive hydrogels in deionized water exhibit high mechanical performances with compressive strength and tensile strength in the range of 7.58-9.52 MPa and 0.48-1.20 MPa respectively

which are ascribed to the intermolecular hydrogen bonding interactions of diaminotriazinediaminotriazine (DAT-DAT) in the network. Meanwhile

adding PEDOT/PSS can significantly increase both the specific conductivities and equilibrium water contents of the hydrogels. These cytocompatible conductive hydrogels may have a great potential to be used as electrical stimuli responsive soft biomaterials.

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references

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