All-Polymer Solar Cells with Perylenediimide Polymer Acceptors

Yi-kun Guo; Yun-ke Li; Han Han; He Yan; Dahui Zhao

doi:10.1007/s10118-017-1893-x

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All-Polymer Solar Cells with Perylenediimide Polymer Acceptors

Papers | Updated：2021-02-18

- All-Polymer Solar Cells with Perylenediimide Polymer Acceptors
- Chinese Journal of Polymer Science Vol. 35, Issue 2, Pages: 293-301(2017)
- Affiliations：
  
  a.Beijing National Laboratory for Molecular Sciences, Center for the Soft Matter Science and Engineering and the Key Laboratory of Polymer Chemistry and Physics of the Ministry of Education, College of Chemistry, Peking University, Beijing 100871, China
  b.Department of Chemistry, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong, China
- Author bio：
  
  He Yan (颜河), E-mail:hyan@ust.hk
  Dahui Zhao (赵达慧), E-mail:dhzhao@pku.edu.cn
- Funds：
- DOI：10.1007/s10118-017-1893-x
  CLC：
- Received：18 October 2016，
  
  Revised：2016-10-31，
  
  Accepted：02 November 2016，
  
  Published：2017-02
- Accepted：
Scan QR Code
Yi-kun Guo, Yun-ke Li, Han Han, et al. All-Polymer Solar Cells with Perylenediimide Polymer Acceptors[J]. Chinese Journal of Polymer Science, 2017, 35(2): 293-301.
DOI：

Yi-kun Guo, Yun-ke Li, Han Han, et al. All-Polymer Solar Cells with Perylenediimide Polymer Acceptors[J]. Chinese Journal of Polymer Science, 2017, 35(2): 293-301. DOI： 10.1007/s10118-017-1893-x.

摘要

Abstract

Four polymers based on perylenediimide co-polymerized with thiophene

bithiophene

selenophone and thieno[3

2-b]thiophene were investigated as the acceptor materials in all-polymer solar cells. Two different donor polymers

poly[4

8-bis (5-(2-ethylhexyl) thiophen-2-yl) benzo[1

2-b; 4

']dithiophene-2

6-diyl-

alt

-(4-(2-ethylhexyl)-3-fluorothieno[3

]thiophene)-2-carboxylate-2

6-diyl]

(PTB7-Th) and poly[(5

6-difluoro-2

3-benzothiadiazol-4

7-diyl)-

alt

-(3

3"'-di (2-dodecyltetradecyl)-2

2';5'

2";5"

2"'-quaterthiophen-5

5"'-diyl)] (PffBT4T-2DT)

with suitably complementary absorption spectra and energy levels were applied and examined. Among all different donor-acceptor pairs studied here

the combination of PTB7-Th:poly[

'-bis (1-hexylheptyl)-3

10-perylenediimide-1

6/1

7-diyl-

alt

-2

5-thiophene] (PDI-Th) exhibited the best power conversion efficiency (PCE) of 5.13%

with open-circuit voltage (

)=0.79 V

short-circuit current density (

)=12.35 mA·cm

-2

and fill-factor (FF)=0.52. The polymer of PDI-Th acceptor used here had a regio-irregular backbone

conveniently prepared from a mixture of 1

6-and 1

7-dibromo-PDI. It is also noteworthy that neither additive nor post-treatment is required for obtaining such a cell performance.

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Keywords

references

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