High Energy Dissipation Polymer Gels by Regulating Relaxation of Confined Chains

Wei Shi; Zong-Zheng Zhang; Ying Li; Chun-Yi Peng; Hao Zha; Jin Huang; Ming-Jie Liu

doi:10.1007/s10118-025-3475-7

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High Energy Dissipation Polymer Gels by Regulating Relaxation of Confined Chains

REVIEW | Updated：2026-02-04

- High Energy Dissipation Polymer Gels by Regulating Relaxation of Confined Chains
- Chinese Journal of Polymer Science Vol. 43, Pages: 1-12(2025)
- Affiliations：
  
  a.State Key Laboratory of Bioinspired Interfacial Materials Science, Center for Bioinspired Science and Technology, Hangzhou International Innovation Institute, Beihang University, Hangzhou 311115, China
  b.Key Laboratory of Bioinspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, China
- Author bio：
  
  huangjin2018@buaa.edu.cn (J.H.)
  liumj@buaa.edu.cn (M.J.L.)
- Funds：
- DOI：10.1007/s10118-025-3475-7
  CLC：
- Received：21 September 2025，
  
  Accepted：08 October 2025，
  
  Published Online：15 January 2026，
  
  Published：2025-12
- Accepted：
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Shi, W.; Zhang, Z. Z.; Li, Y.; Peng, C. Y.; Zha, H.; Huang, J.; Liu, M. J. High energy dissipation polymer gels by regulating relaxation of confined chains. Chinese J. Polym. Sci. https://doi.org/10.1007/s10118-025-3475-7

Wei Shi, Zong-Zheng Zhang, Ying Li, et al. High Energy Dissipation Polymer Gels by Regulating Relaxation of Confined Chains[J/OL]. Chinese Journal of Polymer Science, 2025, 431-12.
Shi, W.; Zhang, Z. Z.; Li, Y.; Peng, C. Y.; Zha, H.; Huang, J.; Liu, M. J. High energy dissipation polymer gels by regulating relaxation of confined chains. Chinese J. Polym. Sci. https://doi.org/10.1007/s10118-025-3475-7 DOI：

Wei Shi, Zong-Zheng Zhang, Ying Li, et al. High Energy Dissipation Polymer Gels by Regulating Relaxation of Confined Chains[J/OL]. Chinese Journal of Polymer Science, 2025, 431-12. DOI： 10.1007/s10118-025-3475-7.

摘要

Composite structure of viscous fluids and elastic skeletons in biological tissues inspired designs of high energy dissipation gels by viscoelastic regulation of networks and confined chains. We summarized progress of damping gels from perspective of network structure

which will promote development of damping polymers towards extreme conditions.

Abstract

Damping polymers relying on significant internal friction in glass transition regions can suppress vibrations and noise; however

these materials generally exhibit a narrow damping breadth and severe mechanical instability. Natural damping tissues such as the skin and cartilage achieve high energy dissipation through the combination of viscous fluid and a 3D elastic skeleton. This binary structure inspired a high energy dissipation gel design strategy using synergistic viscoelastic scheme of confined chains and host network. Herein

we provide a comprehensive overview of recent advances in bio-inspired damping polymer gels. The structural designs and their corresponding performances are elucidated in this review. We anticipate that this review will motivate further exploration of design and applications of damping polymers.

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